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Record W3130981149 · doi:10.21203/rs.3.rs-210447/v1

Tribological interaction of plasma functionalized CaCO3 nanoparticles with zinc and ashless dithiophosphate additives

2021· preprint· en· W3130981149 on OpenAlex
Kimaya Vyavhare, Richard B. Timmons, Ali Erdemir, Pranesh B. Aswath

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueResearch Square · 2021
Typepreprint
Languageen
FieldEngineering
TopicLubricants and Their Additives
Canadian institutionsnot available
FundersArgonne National LaboratoryCanadian Institutes of Health ResearchNatural Sciences and Engineering Research Council of CanadaUniversity of Texas at ArlingtonUniversity of SaskatchewanCanadian Light Source
KeywordsTribologyZincNanoparticlePlasmaMaterials scienceChemical engineeringChemistryMetallurgyNanotechnologyEngineeringPhysics

Abstract

fetched live from OpenAlex

Abstract Surface-modified CaCO 3 nanoparticles, synthesized through plasma-enhanced chemical vapor deposition (PECVD), were employed to improve lubricant additive technology for internal combustion engines via reduction and/or replacement of additives, such as zinc dialkyl dithiophosphate (ZDDP), in engine oil. Various oil formulations were prepared with functionalized CaCO 3 nanoparticles, in combination with ashless dialkyl dithiophosphate (DDP) and ZDDP at low concentrations of phosphorus. Tribological test results indicate synergistic interaction of functionalized CaCO 3 nanoparticles with ZDDP and DDP, providing enhanced friction and wear performance under boundary lubrication. A comparative study of the tribo-surfaces morphology and chemistry was assessed via atomic force microscopy and X-ray absorption near-edge spectroscopy. Improved wear protection by functionalized CaCO 3 BM (borate and methacrylate coated) nanoparticles under boundary lubrication was attributed to the formation of calcium and boron-rich 50–80 nm thick tribofilms on the worn surfaces. XANES results revealed that plasma functionalized CaCO 3 nanoparticles interact with ZDDP and DDP and participate in tribofilm formation through tribo-chemical reactions and metal cation supply to form stable and wear-resistant tribofilms. These results provide strong support for the potential application of plasma functionalized CaCO 3 nano-additives to reduce the concentration of harmful P-based additives in automotive lubricants.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.329
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.056
GPT teacher head0.333
Teacher spread0.277 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it