Americium-241 in peat bogs as a marker of the beginning of the Anthropocene: examples from Europe and North America.
Bibliographic record
Abstract
Americium-241 (241Am) is present in the terrestrial and aquatic environment around the globe as a result of the atmospheric testing of high yield thermonuclear weapons carried out mainly in the 1950s and 1960s. Radioactive debris (including mainly 137Cs, 90Sr, and various Pu isotopes) from the tests was injected high into the stratosphere where it was rapidly dispersed around the world. Over a period of months this material slowly returned to the troposphere, and from there was quickly removed by wet and dry fallout onto the earth’s surface. Amounts of 241Am in freshly deposited weapons test debris were essentially zero. Its presence today is through in-growth from its short-lived precursor 241Pu (half-life 14.4 years). By this process concentrations of 241Am have steadily increased with time and will continue to do so through to around 2040. Widely considered to be immobile in soils and sediments, with its well-known origins and long half-life (432 years), 241Am is in many ways an ideal chronostratigraphic marker of the nuclear age. Calculations show that the 241Am record in any ideal natural archive is a faithful representation of the history of weapons test fallout. Beginning in the early 1950s, fallout reached a peak in 1963 and then declined rapidly following the implementation of the test ban treaty. A number of scientists have proposed that the weapons test fallout peak could be used to mark the start of the Anthropocene. Various geological archives preserve the record of fallout, though with varying degrees of fidelity. They include polar snow and ice, marine and lacustrine sediments, and peat bogs. Bogs are ombrotrophic peatlands in that the plants growing there receive nutrients and contaminants exclusively from the atmosphere. The purpose of this study is to determine the fidelity of 241Am records in peat bog cores. Specifically, we compare the position of the 241Am concentration peak with the 1963 depth determined by 210Pb dating. We use 39 peat cores from Europe, North America, and Indonesia collected by our team during the past 30 years for studies of atmospheric deposition of trace metals, all of which had been independently dated using 210Pb. We find that 18 of the cores provide an excellent agreement between the 241Am and 210Pb dates, 12 were in good agreement, and 9 agreed poorly. Possible reasons for the discrepancy in the 9 cores with the poor agreement are 1) the sensitivity of the gamma spectrometer for detecting 241Am, and 2) disruptions to the fallout records caused e.g. by disturbances to the peat bog or changes in the peat topography or hydrology. Small scale horizontal and vertical variations in bogs help explain why in a triplicate of peat cores collected from Wildseemoor in the Black Forest of Germany, excellent agreement was found in one core, good agreement in a second, and poor agreement in the third. A peat core collected from Gola di Lago, a small fen in Switzerland, showed excellent agreement; this suggests that samples from minerotrophic peatlands may also be useful to mark the start of the Anthropocene.
Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.
How this classification was reachedexpand
Full frame machine prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.
Distilled classifier scores by category (both heads)
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.003 | 0.003 |
| Science and technology studies | 0.001 | 0.001 |
| Scholarly communication | 0.001 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.001 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".