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Dephosphorization Kinetics of Bloated Metal Droplets Reacting with Basic Slag Containing TiO<sub>2</sub>

2021· article· en· W3137239658 on OpenAlexaff
Phillip Brian Drain, Kezhuan Gu, Neslihan Dogan, Raymond J. Longbottom, Michael W. Chapman, Brian J. Monaghan, Kenneth S. Coley

Bibliographic record

VenueISIJ International · 2021
Typearticle
Languageen
FieldEngineering
TopicMetallurgical Processes and Thermodynamics
Canadian institutionsMcMaster University
FundersAustralian Research Council
KeywordsKineticsSlag (welding)SteelmakingChemistryMetalQuenching (fluorescence)Chemical kineticsOxidizing agentReaction rateMaterials scienceMetallurgyChemical engineeringAnalytical Chemistry (journal)ChromatographyFluorescenceCatalysis

Abstract

fetched live from OpenAlex

Although the dephosphorization kinetics of bloated metal droplets reacting with oxidizing slag have been studied in detail in the authors’ laboratory, the mechanism of reaction for slags in a basicity range typical of steelmaking, has been sparsely reported. The current study employed a high temperature furnace equipped with X-ray fluoroscopy to observe the bloating behavior of droplets and tracked dephosphorization kinetics by quenching and analyzing droplets after different reaction times. The mechanism of reaction between bloated metal droplets and slag was studied at 1923 K for slags with basicity range C/S=2.56. The rate and extent of dephosphorization was found to be greater in CMS slags compared to CAS slags due to the faster mass transport and a larger thermodynamic driving force. The kinetic analysis showed that the reaction proceeded in two distinct stages, a fast initial stage followed by a slower stage. The km during the first stage of dephosphorization was at least 8 times higher than that during the second stage. This is proposed to be due to a higher internal CO generation rate during the initial stage which increases the rate of surface renewal. The effect of TiO2 on dephosphorization kinetics was also investigated in terms of thermodynamic driving force.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.199
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2021
Admission routes1
Has abstractyes

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