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Record W3142221362 · doi:10.1038/s42005-022-00901-7

Field-induced quantum critical point in the itinerant antiferromagnet Ti3Cu4

2022· article· en· W3142221362 on OpenAlexafffund
Jaime M. Moya, Alannah M. Hallas, Vaideesh Loganathan, C.-L. Huang, Lazar Kish, A. A. Aczel, J. Beare, Yipeng Cai, G. M. Luke, Franziska Weickert, Andriy H. Nevidomskyy, Christos D. Malliakas, Mercouri G. Kanatzidis, Shiming Lei, Kyle Bayliff, E. Morosan

Bibliographic record

VenueCommunications Physics · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicRare-earth and actinide compounds
Canadian institutionsTRIUMFMcMaster UniversityUniversity of British Columbia
FundersOak Ridge National LaboratoryKavli Institute for Theoretical Physics, University of California, Santa BarbaraArgonne National LaboratoryU.S. Department of EnergyInternational Institute for Nanotechnology, Northwestern UniversityDivision of Electrical, Communications and Cyber SystemsBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaDivision of Materials ResearchOffice of ScienceNorthwestern UniversityNational High Magnetic Field LaboratoryWelch FoundationHigh Magnetic Field Laboratory, Chinese Academy of SciencesTRIUMFNational Science Foundation
KeywordsCondensed matter physicsQuantum critical pointMagnetismAntiferromagnetismPhysicsMagnetic momentQuantum phase transitionPhase transition

Abstract

fetched live from OpenAlex

Abstract New phases of matter emerge at the edge of magnetic instabilities, which can occur in materials with moments that are localized, itinerant or intermediate between these extremes. In local moment systems, such as heavy fermions, the magnetism can be tuned towards a zero-temperature transition at a quantum critical point (QCP) via pressure, chemical doping, and, rarely, magnetic field. By contrast, in itinerant moment systems, QCPs are more rare, and they are induced by pressure or doping; there are no known examples of field induced transitions. This means that no universal behaviour has been established across the whole itinerant-to-local moment range—a substantial gap in our knowledge of quantum criticality. Here we report an itinerant antiferromagnet, Ti3Cu4, that can be tuned to a QCP by a small magnetic field. We see signatures of quantum criticality and the associated non-Fermi liquid behaviour in thermodynamic and transport measurements, while band structure calculations point to an orbital-selective, spin density wave ground state, a consequence of the square net structural motif in Ti3Cu4. Ti3Cu4 thus provides a platform for the comparison and generalisation of quantum critical behaviour across the whole spectrum of magnetism.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.049
GPT teacher head0.327
Teacher spread0.277 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2022
Admission routes2
Has abstractyes

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