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Record W3148471444 · doi:10.1088/1361-648x/abf594

Magnetic ordering in the Ising antiferromagnetic pyrochlore Nd <sub>2</sub> ScNbO <sub>7</sub>

2021· article· en· W3148471444 on OpenAlexafffund
Cole Mauws, Nathaniel Hiebert, Megan Rutherford, Haidong Zhou, Qing Huang, M. B. Stone, Nicholas P. Butch, Yixi Su, Eun Sang Choi, Z. Yamani, C. R. Wiebe

Bibliographic record

VenueJournal of Physics Condensed Matter · 2021
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsMcMaster UniversityUniversity of WinnipegNational Research Council CanadaUniversity of Manitoba
FundersOak Ridge National LaboratoryNational Research Council CanadaOffice of ScienceCanada Research ChairsNational Science FoundationCanadian Institutes of Health ResearchDivision of Materials ResearchNational Institute of Standards and TechnologyLeverhulme TrustCanada Foundation for InnovationCanadian Institute for Advanced ResearchNatural Sciences and Engineering Research Council of CanadaCanadian Light SourceNational High Magnetic Field LaboratoryU.S. Department of Energy
KeywordsAntiferromagnetismPyrochloreCondensed matter physicsMagnetismSpin glassInelastic neutron scatteringNeodymiumIsing modelSymmetry breakingNeutron scatteringExcited stateSpin wavePhysicsScatteringFerromagnetismAtomic physicsOpticsQuantum mechanics

Abstract

fetched live from OpenAlex

Abstract The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behaviour, here we describe a system in which the structural disorder results in long-range antiferromagnetic order due to local symmetry breaking. Nd 2 ScNbO 7 is shown to have a dispersionless gapped excitation observed in other neodymium pyrochlores below T N = 0.37 K through polarized and inelastic neutron scattering. However the dispersing spin waves are not observed. This excited mode is shown to occur in only 14(2)% of the neodymium ions through spectroscopy and is consistent with total scattering measurements as well as the magnitude of the dynamic moment 0.26(2) μ B . The remaining magnetic species order completely into the all-in all-out Ising antiferromagnetic structure. This can be seen as a result of local symmetry breaking due disordered Sc +3 and Nb +5 ions about the A -site. From this work, it has been established that B -site disorder restores the dipole-like behaviour of the Nd +3 ions compared to the Nd 2 B 2 O 7 parent series.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.082
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.226
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2021
Admission routes2
Has abstractyes

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