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Record W3151576209 · doi:10.1016/j.enceco.2021.03.003

Novel aluminium (hydr) oxide-functionalized activated carbon derived from Raffia palm (Raphia hookeri) shells: Augmentation of its adsorptive properties for efficient fluoride uptake in aqueous media

2021· article· en· W3151576209 on OpenAlexaff
Raphael Terungwa Iwar, Oliver Terna Iorhemen, Kola Ogedengbe, Kamil Kayode Katibi

Bibliographic record

VenueEnvironmental Chemistry and Ecotoxicology · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicFluoride Effects and Removal
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsAdsorptionFluorideActivated carbonLangmuir adsorption modelNuclear chemistryMaterials scienceAqueous solutionFourier transform infrared spectroscopyChemical engineeringChemistryInorganic chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

In this study a novel activated carbon derived from Raffia palm shells was synthesized firstly by activating the precursor with phosphoric acid to produce Raffia Palm Shell Activated Carbon (RPSAC) and further functionalized by coating its surface with aluminium hydroxide to produce a composite called Aluminium Oxide-coated Raffia Palm Shell Activated Carbon (ACRPSAC). These adsorbents were extensively characterized and tested for fluoride adsorption in aqueous media using batch adsorption experiment in comparison with a commercially available activated carbon (CAC). ACRPSAC demonstrated excellent qualities and fluoride adsorption capacity as compared to RPSAC. SEM/EDX revealed that ACRPSAC developed both micro and meso-pores on its surface with BET-surface area and pore volume of 715.80 m2/g and 0.47 cm3/g respectively. FTIR and XRD proved that ACRPSAC was largely amorphous and had sufficient functionality for fluoride uptake in solution. Batch adsorption studies showed that the fluoride removal abilities were in the order of ACRPSAC > RPSAC > CAC with maximum Langmuir adsorption capacity of 4.10 > 2.26 > 2.24 mg/g. respectively. The experimental data was well described by the Langmuir (R2 = 0.8802–0.9751) and the pseudo-second order kinetic (R2 = 0.9974–0.9999) models, signifying that fluoride uptake by the adsorbents was a chemisorption process. Thermodynamic studies revealed that the process was spontaneous, endothermic and feasible for ACRPSAC and RPSAC but was non-spontaneous for CAC. It was concluded that ACRPSAC is an excellent activated carbon for eliminating fluoride from groundwater and can be further studied for its commercialization.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.196
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations35
Published2021
Admission routes1
Has abstractyes

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