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Record W3161019398 · doi:10.1002/adsu.202100054

On the Investigation of the Thermal Degradation of Waste Printed Circuit Boards for Recycling Applications

2021· article· en· W3161019398 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAdvanced Sustainable Systems · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicRecycling and Waste Management Techniques
Canadian institutionsUniversité de MontréalPolytechnique Montréal
Fundersnot available
KeywordsThermogravimetric analysisPyrolysisThermochemistryElectronic wasteDifferential scanning calorimetryChemical engineeringDegradation (telecommunications)Printed circuit boardFire retardantPolymerCeramicMaterials scienceEvolved gas analysisThermal analysisChemistryWaste managementThermalOrganic chemistryInorganic chemistryComputer science

Abstract

fetched live from OpenAlex

Abstract Electronic products contain a wide range of materials including pure metals and alloys, ceramics, and polymers. Disassembling each individual component of such products to recycle is impossible. For that reason, end‐of‐life electronic products like waste printed circuit boards (WPCB) are shredded and sent to pyrometallurgical processes to recover valuable metals. One major issue with recycling is the release of gaseous brominated species that need to be captured or stabilized. It is crucial to have a fundamental understanding of the chemical interactions that occur between each component of the WPCB in these processes. The thermal degradation mechanism of WPCB is investigated here using differential scanning calorimetry coupled to thermogravimetric analysis of both synthetic samples and shredded WPCB. Computational thermochemistry is used to support the identified reaction mechanisms which involve the release of gaseous hydrogen bromide evolving from Tetrabromobisphenol A used as a flame retardant. The chemical reactivity between this compound and each major WPCB component is quantified. It is proven that HBr(g) reacts with copper, iron, and CaO to form bromides which stay in the solid pyrolysis residue up to a temperature of 580 °C. Above this temperature, CuBr 2 and FeBr 2 start to evaporate and are lost in the gas phase.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.604
Threshold uncertainty score0.220

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.232
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it