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Record W3164713056 · doi:10.1021/acsomega.1c01800

Experimental Simulation of Hydrocarbon Expulsion in Semi-open Systems from Variable Organic Richness Source Rocks

2021· article· en· W3164713056 on OpenAlexaff
Lianhua Hou, Haiping Huang, Chun Yang, Weijiao Ma

Bibliographic record

VenueACS Omega · 2021
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of Calgary
FundersNational Natural Science Foundation of China
KeywordsSource rockTotal organic carbonMaturity (psychological)Oil shaleHydrocarbonVitrinite reflectanceMineralogyGeologyChemistryStructural basinEnvironmental chemistryGeomorphologyPaleontologyOrganic chemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide To better understand oil and gas generation and expulsion mechanisms and their controlling factors, two-stage heating program (20 and 5 °C/d) at 11 target temperatures (250–580 °C) have been performed in a semi-open reactor on nine immature lacustrine shale samples from the Triassic Yanchang Formation in Ordos Basin, NW China, with total organic carbon (TOC) contents ranging from 0.5% to 30.0%. The cumulative expelled oil and gas were quantified and correlated with the measured vitrinite reflectance (% R o ) and residual TOC. The amount of expelled oil increases substantially with increasing maturity in the R o range of 0.5–1.25% and ends at R o of >1.45%, while the volume of expelled gas increases markedly with maturity when R o is >1.0%. Organic richness exerts primary control on the expulsion yields, which increase linearly with increasing original TOC (TOC o ) per unit weight of rock, whereas the increment decreases with TOC o per unit weight of TOC, once the TOC o content is above 5%. Marked TOC reduction occurs in the R o of 0.5–1.1% due to oil generation and expulsion, but the trend is reversed in the higher maturity range possibly caused by the simultaneous decomposition of minerals. Numerical correlations among heating temperatures, % R o, TOC content, and expelled oil and gas yields have been constructed, and the minimum TOC contents for effective oil and gas source rocks have been inferred. The lowest TOC contents of 0.5% and 0.48% are required for oil and gas expulsion in the oil and gas generation window, corresponding to the TOC o of 0.91% and 0.76%, respectively. The minimum TOC content for effective gas source rocks decreases slightly with increasing maturity; however, a much higher TOC cutoff is required for lower maturity level source rocks. Wide range of TOC content variation in our studied samples provides well constraint of organic richness on oil and gas generation and expulsion behaviors and their evolution trajectory during thermal evolution, which will fascinate source rock quality and exploration potential assessment in other source rock systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.065
Threshold uncertainty score0.602

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.238
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2021
Admission routes1
Has abstractyes

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