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Record W3171115315 · doi:10.1038/s41598-021-91301-4

Spin polarized density functional theory calculations of the electronic structure and magnetism of the 112 type iron pnictide compound $$\hbox {EuFeAs}_2$$

2021· article· en· W3171115315 on OpenAlexafffund
Farshad Nejadsattari, Z. M. Stadnik

Bibliographic record

VenueScientific Reports · 2021
Typearticle
Languageen
FieldMaterials Science
TopicIron-based superconductors research
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsDensity functional theoryMagnetic momentMagnetismIsostructuralCondensed matter physicsElectronic structureAtom (system on chip)Hyperfine structureFermi levelChemistryIonic bondingDensity of statesValence (chemistry)Chemical bondPhysicsAtomic physicsCrystallographyElectronComputational chemistryCrystal structureQuantum mechanicsIon

Abstract

fetched live from OpenAlex

Using density-functional theory, we investigate the electronic, magnetic, and hyperfine-interaction properties of the 112-type iron-pnictide compound [Formula: see text], which is isostructural to the high-temperature iron-based superconductor [Formula: see text]. We show that the band structure of [Formula: see text] is similar to that of the 112-type compounds' family, with hole-like and electron-like bands at the Brillouin-zone center and corners, respectively. We demonstrate that the bands near the Fermi level originate mainly from the Fe atoms. The presence of a mixture of ionic and covalent bonding is predicted from the charge-density and atom-resolved density-of-states calculations. There is good agreement between the calculated hyperfine-interaction parameters with those obtained from the [Formula: see text]Fe and [Formula: see text]Eu Mössbauer measurements. The spatial distribution of atoms in [Formula: see text] leads to an in-plane 2D magnetism. Moreover, ab-initio calculations predict the compound's magnetic moment and the magnetic moments of each constituent atom. Also, the density of states profile provides insight into the relative magnitude of these moments. Electronic structure calculations and Fermi surface topology reveal various physical and chemical properties of [Formula: see text]. Valence electron density maps indicate the co-existence of a wide range of chemical bonds in this system, and based on structural properties, the transport characteristics are deduced and discussed. A thorough analysis of the atomic structure of [Formula: see text] and its role in the bond formation is presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.125
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.250
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2021
Admission routes2
Has abstractyes

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