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Record W3176983082 · doi:10.1002/smll.202100323

Recent Development of Electrocatalytic CO<sub>2</sub> Reduction Application to Energy Conversion

2021· review· en· W3176983082 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueSmall · 2021
Typereview
Languageen
FieldEnergy
TopicCO2 Reduction Techniques and Catalysts
Canadian institutionsWestern University
FundersNational Key Research and Development Program of ChinaNational Natural Science Foundation of China
KeywordsFaraday efficiencyElectrochemistryMaterials scienceCarbon fibersGreenhouse gasElectricity generationTransition metalEnergy transformationElectricityNanotechnologyProcess (computing)Process engineeringCatalysisChemistryComputer scienceElectrodeEngineeringOrganic chemistryPower (physics)

Abstract

fetched live from OpenAlex

Abstract Carbon dioxide (CO 2 ) emission has caused greenhouse gas pollution worldwide. Hence, strengthening CO 2 recycling is necessary. CO 2 electroreduction reaction (CRR) is recognized as a promising approach to utilize waste CO 2 . Electrocatalysts in the CRR process play a critical role in determining the selectivity and activity of CRR. Different types of electrocatalysts are introduced in this review: noble metals and their derived compounds, transition metals and their derived compounds, organic polymer, and carbon‐based materials, as well as their major products, Faradaic efficiency, current density, and onset potential. Furthermore, this paper overviews the recent progress of the following two major applications of CRR according to the different energy conversion methods: electricity generation and formation of valuable carbonaceous products. Considering electricity generation devices, the electrochemical properties of metal–CO 2 batteries, including Li–CO 2 , Na–CO 2 , Al–CO 2 , and Zn–CO 2 batteries, are mainly summarized. Finally, different pathways of CO 2 electroreduction to carbon‐based fuels is presented, and their reaction mechanisms are illustrated. This review provides a clear and innovative insight into the entire reaction process of CRR, guiding the new electrocatalysts design, state‐of‐the‐art analysis technique application, and reaction system innovation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.991
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.278
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it