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Record W3184483668

Electrokinetic-Induced Phase Separation of Petroleum Wastes: Evaluation of Oil Sediment Behavior and Solids Properties

2020· dissertation· en· W3184483668 on OpenAlexfundno aff
Esmaeel Kariminezhad

Bibliographic record

VenueSpectrum Research Repository (Concordia University) · 2020
Typedissertation
Languageen
FieldEngineering
TopicElectrokinetic Soil Remediation Techniques
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaConcordia UniversitySuncor Energy Incorporated
KeywordsElectrokinetic phenomenaPetroleumPhase (matter)Current (fluid)Materials scienceWettingSedimentSeparation processAnodeChemical engineeringEnvironmental scienceChemistryChromatographyNanotechnologyGeologyComposite materialEngineering
DOInot available

Abstract

fetched live from OpenAlex

The disposal of the oily wastes represents a serious threat to the environment. The treatment of such oily wastes poses significant challenges considering their physical and chemical properties. This study focuses on advanced electrokinetic methods as a technology to treat oily sediments through phase separation. The study comprises four objectives which are intimately linked to achieve the overall objective of exploring the electrokinetic method for treatment of water-in-oil emulsions. The first objective is finding the most efficient oil phase separation when four different regimes of electric fields are applied (namely constant direct current (CDC), pulsed direct current (PDC), incremental direct current (IDC) and decremental direct current (DDC)). The second objective is to investigate the factors affecting the electrokinetic process and dewaterability of different types of oily sludge. The third objective is investigating the effect of nanoparticles and synthesized catalysts on the phase separation efficiency within the electrokinetic system. The final objective was to elucidate the various mechanisms underlying the separation of oil, water and solids by thermal analysis of treated samples. 
\nThe results showed that the extent and quality of phase separation depend on the regime of electrical current applied. The DDC and IDC regimes resulted in the most efficient phase separation of the oil sediments, and even incurred a highly resolved separation of light hydrocarbons at the top anode. 
\nX-ray photoelectron spectroscopy (XPS) analyses showed a decrease in the concentration of carbon from 99% in centrifuged samples to 63% on the surface of the solids treated by PDC. Wettability alteration studies showed an increase in the level of fine solids in the aqueous phase following electrokinetic treatment thereby enhancing the hydrophilicity of the solids. 
\nThe best performance of titanium dioxide (TiO2) nanoparticles and a synthesized catalyst reactors results were obtained with the synthesized catalyst as compared to the use of TiO2 nanoparticles. Activation energy emphasized the effect of additives on separation of phases and availability of oil. Hence, the synergistic effects of TiO2 or synthesized catalyst with electrokinetic treatment can lead to better phase separation and may reinforce the current applications of the electrokinetic method in treating oil sediments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.024
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.314
Teacher spread0.274 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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