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Record W3187011914 · doi:10.1088/1361-6528/ac1753

Synthesis, characterization, and visible light photocatalytic activity of solution-processed free-standing 2D Bi <sub>2</sub> O <sub>2</sub> Se nanosheets

2021· article· en· W3187011914 on OpenAlexafffund
Damini Vrushabendrakumar, Harshitha Rajashekhar, Saralyn Riddell, Aarat P. Kalra, Kazi M. Alam, Karthik Shankar

Bibliographic record

VenueNanotechnology · 2021
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsNational Institute for NanotechnologyUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCanada First Research Excellence FundAlberta Innovates
KeywordsPhotocatalysisMaterials scienceBismuthVisible spectrumBand gapChemical engineeringDegradation (telecommunications)NanotechnologyOptoelectronicsCatalysisOrganic chemistryElectronic engineeringMetallurgy

Abstract

fetched live from OpenAlex

Abstract Owing to their unique structural and electronic properties such as layered structure with tuneable bandgap and high electron mobility, 2D materials have emerged as promising candidates for photocatalysis. Recently, bismuth oxyselenide (Bi 2 O 2 Se), a member of bismuth oxychalcogenide’s family has shown great potential in high-speed field-effect transistors, infrared photodetectors, ferroelectric devices, and electrochemical sensors. However, the potential of Bi 2 O 2 Se in photocatalysis has not yet been explored. In the current work, Bi 2 O 2 Se nanosheets with an average size of ∼170 nm and a lattice strain of 0.01 were synthesized at room temperature using a facile solution-processed method and the as-synthesized material was investigated with various characterization techniques such as x-ray diffraction, FE-SEM, UV–vis spectroscopy. The bandgap for the indirect transition in Bi 2 O 2 Se nanosheets was estimated to be 1.19 eV. Further, the visible-light-driven photocatalytic degradation of methylene blue (MB) dye using Bi 2 O 2 Se as a photocatalyst is presented. The photocatalytic experiments demonstrate the promising photocatalytic ability of Bi 2 O 2 Se as it leads to 25.06% degradation of MB within 80 min of light illumination. The effect of active species trapping agents (carrier and radical scavengers) on photocatalytic activity is also presented and discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.232
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations27
Published2021
Admission routes2
Has abstractyes

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