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Record W3189171423 · doi:10.1007/s12665-021-09959-y

Occurrence and characterisation of naphthenic acid fraction components in oil residues and sediments stranded on the shoreline of Chedabucto Bay, Nova Scotia, Canada

2021· article· en· W3189171423 on OpenAlexafffundabout
Zeyu Yang, Gong Zhang, Chun Yang, Keval Shah, Bruce P. Hollebone, Sonia Laforest, Patrick Lambert, Carl E. Brown, Jane Situ, Alexandra Verkuyl

Bibliographic record

VenueEnvironmental Earth Sciences · 2021
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsEnvironment and Climate Change Canada
FundersGovernment of Canada
KeywordsNaphthenic acidBayEnvironmental chemistryNova scotiaSedimentEnvironmental sciencePetroleumAbundance (ecology)ChemistryOceanographyGeologyEcologyBiology

Abstract

fetched live from OpenAlex

Abstract In June 2016, oil residues and sediment samples were collected from the shoreline of Chedabucto Bay, Nova Scotia, Canada, at sites affected by the 1970 Arrow oil spill. This study aimed to investigate the occurrence, fate, and behaviour of oil components 45 years post-spill by analysing polar naphthenic acid fraction components (NAFCs) through high-performance liquid chromatography–high-resolution mass spectrometry (HPLC–HRMS). In all samples, the most abundant NAFC species were those having only oxygen as the heteroatom ( O o species, o indicating the number of oxygen atoms, from 1 to 8) and a high degree of saturation. NAFC species only containing two oxygen atoms (O 2 ) accounted for 50–70% of all O o species. The abundance of all remaining species was negligible compared with O o species. NAFCs in most Arrow oil residues had higher levels of oxygen species than the oil remaining stored in the sunken tanker. Environmental sediment samples collected from near a marina away from the spill site contained a dominant biological, whereas all Arrow oil residues were mainly composed of NAFCs that are characteristic of petroleum. The abundance of NAFCs in the Arrow oil residues varied between sites, confirming that site-specific environmental conditions play a major role in controlling the fate and behaviour of oil components, including NAFCs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.132
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.222
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2021
Admission routes3
Has abstractyes

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