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Record W3191159231 · doi:10.14288/1.0401265

A numerical description of nitrogen diffusion in titanium at elevated temperatures

2021· article· en· W3191159231 on OpenAlexaff
Daniel Hawker

Bibliographic record

VenuecIRcle (University of British Columbia) · 2021
Typearticle
Languageen
FieldMaterials Science
TopicFusion materials and technologies
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsNitrogenDiffusionTitaniumMaterials scienceThermodynamicsMathematicsChemistryMetallurgyPhysics

Abstract

fetched live from OpenAlex

As part of a program to understand the dissolution of nitrogen-rich titanium solids in liquid titanium, a numerical study of nitrogen diffusion in titanium at elevated temperatures has been carried out. A Landau transformation was applied to the equations governing nitrogen diffusion which were used as the basis for the numerical models developed in this study. To begin a numerical model describing the nitriding of commercially pure titanium was developed. The numerical model was used initially to simulate nitrogen diffusion in a planar geometry and the predicted nitrogen concentration profiles and displacement of Ti-N phase boundaries showed good agreement with analytically derived solutions. The numerical model was then used to simulate nitrogen transport in commercially pure titanium cylinders. The model results were shown to be sensitive to the diffusion coefficients of Ti-N phases present in the system. Based on a sensitivity analysis, diffusion coefficients at 1650 °C of 4.3×10⁻¹¹ m²·s⁻¹, 1.6×10⁻¹¹ m²·s⁻¹ and 1.7×10⁻¹² m²·s⁻¹ for β-Ti, α-Ti and TiN phases, respectively, were back calculated using the model. The model predictions, using the new diffusion coefficients, showed good agreement with previously published data in terms of both the nitrogen concentration profiles and displacements of Ti-N phase boundaries under the conditions examined in the study. The comparison indicates the model framework is capable of accurately approximating the diffusion of nitrogen in titanium at elevated temperatures. In work that followed, the model framework was used to develop an improved numerical model for describing the dissolution of Ti-N particles in liquid titanium. The results of the improved methodology have been compared to a second finite-difference based model formulated using the conventional approach for interface motion. The improved approach accurately accounts for conservation of nitrogen associated with interface motion and hence has the potential to predict particle dissolution times more accurately in commercial melt refining operations.

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How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.947
Threshold uncertainty score0.975

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.172
Teacher spread0.163 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2021
Admission routes1
Has abstractyes

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