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Record W3192786521 · doi:10.1021/acs.jpclett.1c01856

Theoretical Understanding of Structure–Property Relationships in Luminescence of Carbon Dots

2021· review· en· W3192786521 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Journal of Physical Chemistry Letters · 2021
Typereview
Languageen
FieldMaterials Science
TopicCarbon and Quantum Dots Applications
Canadian institutionsUniversity of Calgary
FundersNatural Science Foundation of Henan ProvinceChina Postdoctoral Science FoundationNational Natural Science Foundation of China
KeywordsLuminescenceMaterials scienceProperty (philosophy)Quantum dotNanotechnologyPhosphorescenceCarbon fibersOptoelectronicsEngineering physicsFluorescencePhysicsOptics

Abstract

fetched live from OpenAlex

Carbon dots (CDs) have excellent luminescence characteristics, such as good light stability, high quantum yield (QY), long phosphorescence lifetime, and a wide emission wavelength range, resulting in CDs' great success in optical applications. Understanding the structure-property relationships in CDs is essential for their use in optoelectronic applications. However, because of the complex nature of CD structures and synthesis processes, understanding the luminescence mechanism and structure-property relationships of CDs is a big challenge. This Perspective reviews the theoretical efforts toward the understanding of structure-property relationships and discusses the challenges that need to be overcome in future development of CDs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.467
Threshold uncertainty score0.439

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.057
GPT teacher head0.299
Teacher spread0.243 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it