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Record W3193395483 · doi:10.1016/j.jmrt.2021.08.047

Sustainable synthesis of multiple-metal-doped Fe2O3 nanoparticles with enhanced photocatalytic performance from Fe-bearing dust

2021· article· en· W3193395483 on OpenAlexaff
Nan Li, Yan Jiang, Yunlong He, Lei Gao, Zhongzhou Yi, Fengrui Zhai, Kinnor Chattopadhyay

Bibliographic record

VenueJournal of Materials Research and Technology · 2021
Typearticle
Languageen
FieldEnergy
TopicIron oxide chemistry and applications
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsPhotocatalysisMaterials scienceMethyl orangeAqueous solutionPhotodegradationNanoparticleScanning electron microscopeNuclear chemistryVisible spectrumPrecipitationLeaching (pedology)Chemical engineeringNanotechnologyComposite materialCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

An Fe-abundant solid waste, fabric filter dust (FFD) was used as the starting material for the preparation of metal-doped Fe2O3 (M−Fe2O3) nanoparticles for the photocatalytic degradation of MO aqueous solution. Valuable elements including Fe, Ti, Al, Na, Si, Ca, and Mg were extracted from the dust by hydrochloric acid leaching, transformed into sediments by increasing the pH of the lixivium orderly, and converted into M−Fe2O3 nanoparticles by the sol–gel technology. The effects of pH for the precipitation process and firing temperature for the sol–gel method were investigated systematically. The M−Fe2O3 samples were characterised using X-ray diffraction, field emission scanning electron microscopy, Brunauer–Emmett–Teller analysis, UV–vis spectra, and energy dispersive spectroscopy. The performances of the dust-derived nanoparticles during photocatalytic process were appraised by visible light photodegradation of methyl orange (MO) aqueous solution, indicating that the M−Fe2O3 (M = Ti and Al) sample prepared with a precipitation pH of 4 and a firing temperature of 500 °C exhibits the most impressive photocatalytic behaviour. The product produces a degradation rate of 82.99% for 100 mL of MO solution (10 mg/L) after visible-light degradation for 180 min, which is increased from 38.94% achieved by an undoped Fe2O3 sample prepared under the same conditions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.303

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.275
Teacher spread0.253 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2021
Admission routes1
Has abstractyes

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Same venueJournal of Materials Research and TechnologySame topicIron oxide chemistry and applicationsFrench-language works237,207