MétaCan
Menu
Back to cohort
Record W3193844673 · doi:10.3390/app11062672

Electrifying with High-Temperature Water Electrolysis to Produce Syngas from Wood via Oxy-Gasification, Leading to Superior Carbon Conversion Yield for Methanol Synthesis

2021· article· en· W3193844673 on OpenAlexaff
Sylvain Larose, Raynald Labrecque, Patrice Mangin

Bibliographic record

VenueApplied Sciences · 2021
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsHydro-QuébecUniversité du Québec à Trois-Rivières
Fundersnot available
KeywordsSyngasWater-gas shift reactionWaste managementFossil fuelSynthetic fuelCarbon fibersGreenhouse gasWood gas generatorMethanolBiofuelIntegrated gasification combined cycleSyngas to gasoline plusYield (engineering)Environmental sciencePulp and paper industryHydrogen productionSteam reformingChemistryCoalMaterials scienceHydrogenCatalysisOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Due to concerns regarding fossil greenhouse gas emissions, biogenic material such as forest residues is viewed nowadays as a valuable source of carbon atoms to produce syngas that can be used to synthesise biofuels such as methanol. A great challenge in using gasified biomass for methanol production is the large excess of carbon in the syngas, as compared to the H2 content. The water–gas shift (WGS) reaction is often used to add H2 and balance the syngas. CO2 is also produced by this reaction. Some of the CO2 has to be removed from the gaseous mixture, thus decreasing the process carbon yield and maintaining CO2 emissions. The WGS reaction also decreases the overall process heat output. This paper demonstrates the usefulness of using an extra source of renewable H2 from steam electrolysis instead of relying on the WGS reaction, for a much higher performance of syngas production from gasification of wood in a simple system with a fixed-bed gasifier. A commercial process simulation software is employed to predict that this approach will be more efficient (overall energy efficiency of about 67%) and productive (carbon conversion yield of about 75%) than relying on the WGS reaction. The outlook for this process that includes the use of the solid oxide electrolyser technology appears to be very promising because the electrolyser has the dual function of providing all of the supplemental H2 required for syngas balancing and all the O2 required for the production of a suitable hot raw syngas. This process is conducive to biomethanol production in dispersed, small plants using local biomass for end-users from the same geographical area, thus contributing to regional sustainability.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.815

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.222
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2021
Admission routes1
Has abstractyes

Explore more

Same venueApplied SciencesSame topicCatalysts for Methane ReformingFrench-language works237,207