MétaCan
Menu
Back to cohort
Record W3195463611 · doi:10.1016/j.sajce.2021.08.004

Optimal removal of diclofenac and amoxicillin by activated carbon prepared from coconut shell through response surface methodology

2021· article· en· W3195463611 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueSouth African Journal of Chemical Engineering · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsInstitut National de la Recherche Scientifique
Fundersnot available
KeywordsAdsorptionActivated carbonChemistryLangmuir adsorption modelNuclear chemistryResponse surface methodologyAqueous solutionDiclofenac SodiumMicroporous materialIodine valueCarbon fibersPhosphoric acidChromatographyOrganic chemistryMaterials scienceComposite material

Abstract

fetched live from OpenAlex

Agricultural residues like coconut shell are widely available in Benin Republic and can be used as adsorbent. In this study, we determine the limits of pharmaceutical substances adsorption by activated carbon from coconut shells. The synthesis of this adsorbent was optimized by the Response Surface Methodology (RSM) with two factors: the impregnation ratio IR and activation temperature. The iodine value was considered as the performance (response) parameter of this synthesis. After characterizing the prepared activated carbon, adsorption tests were performed on diclofenac sodium (DCF) and amoxicillin (AMX) by varying the contact time and the adsorbate-adsorbent ratio Rads. The synthesis results showed that the optimal physicochemical properties of the activated carbon were observed at 740 °C with phosphoric acid (IR = 1.66). Under these optimal conditions, the activated carbon from the coconut shells presented a large microporous specific surface (SBET = 437 m2/g and Vmicro = 0.21 cm3/g), optimal iodine adsorption (930.28 mg/g), amorphous and low heterogeneous chemical composition. In addition, the prepared activated carbon was an excellent adsorbent for the removal of the pharmaceutical substances studied. The experimental adsorption data followed the Langmuir isotherm and the pseudo first-order kinetic model. However, the efficiency varied depending on the nature of the adsorbate and the adsorbate-adsorbent ratio was the main limiting factor in the adsorption process. Optimal elimination greater than 98% was noticed with Rads = 0.10 and a contact time of 15 min (90 min) for DCF (AMX). However, we noticed the complete elimination of AMX (DCF) for Rads ≤ 0.075 (Rads ≤ 0.040). It was observed that the removal efficiency of pollutant was not defined by the adsorption rate constant but the reactivity with the adsorbent.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.062
Threshold uncertainty score0.590

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.225
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it