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Record W3196194050 · doi:10.1002/elsa.202100029

Innovative approach for the synthesis of graphene/MnO<sub>2</sub> nanocomposites and their electrochemical behavior

2021· article· en· W3196194050 on OpenAlexaff
Benjamin D. Ossonon, Ana C. Tavares

Bibliographic record

VenueElectrochemical Science Advances · 2021
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsInstitut National de la Recherche Scientifique
Fundersnot available
KeywordsGrapheneMaterials scienceExfoliation jointSupercapacitorRaman spectroscopyNanocompositeThermogravimetric analysisX-ray photoelectron spectroscopyChemical engineeringElectrodeScanning electron microscopeElectrochemistryComposite numberManganeseNanoparticleTransmission electron microscopyNanotechnologyComposite materialChemistryMetallurgy

Abstract

fetched live from OpenAlex

Abstract Graphene‐manganese dioxide composites were prepared using a simple one step method consisting of the electrochemical exfoliation of graphite in the presence of KMnO 4 in 0.1 м H 2 SO 4 at low temperature . In these conditions, the freshly exfoliated graphene sheets (EG) spontaneously reduce the permanganate ions and EG sheets decorated with MnO 2 nanoparticles are obtained. This was confirmed by scanning electron microscopy coupled with energy dispersive X‐ray spectroscopy, transmission electron microscopy, X‐ray diffraction, Raman, and X‐ray photoelectron spectroscopies and thermogravimetric analysis. The electrochemical properties of EG@MnO 2 material were investigated and discussed. Electrodes based on the composite material exhibited enhanced capacitive performances compared to those made from pure graphene sheets. This was attributed to the synergic effect between the two components (graphene sheets and manganese dioxide nanoparticles) and to a larger porosity of the EG@MnO 2 electrode compared to the EG electrode. Additionally, over 91.6% of original capacitance was retained after 4000 cycles, indicating a very good cycling capability of the composite material. Remarkably, the composite electrode showed promising properties in aqueous medium by exhibiting a large and stable operating voltage up 2 V. The results presented in this article could serve as a guide for improving the energy density of supercapacitors in aqueous media.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.524

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.236
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2021
Admission routes1
Has abstractyes

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