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Record W3196272632 · doi:10.1038/s41597-021-01002-w

Inter-laboratory mass spectrometry dataset based on passive sampling of drinking water for non-target analysis

2021· article· en· W3196272632 on OpenAlexfundno aff
Bastian Schulze, Denice van Herwerden, Ian Allan, Lubertus Bijlsma, Néstor Etxebarría, Martin Hansen, Sylvain Merel, Branislav Vrana, Reza Aalizadeh, B. L. Bajema, Florian Dubocq, Gianluca Coppola, Aurélie Fildier, Pavla Fialová, Emil Egede Frøkjær, Roman Grabic, Pablo Gago-Ferrero, Thorsten Klaus Otto Gravert, Juliane Hollender, Nina Huynh, Griet Jacobs, Tim Jonkers, Sarit Kaserzon, M.H. Lamoree, Julien Le Roux, Teresa Mairinger, C. Margoum, G. Máscolo, Emmanuelle Mebold, Frank Menger, Cécile Miège, Jeroen Meijer, Régis Moilleron, Sapia Murgolo, Massimo Peruzzo, Martijn Pijnappels, Malcolm J. Reid, Claudio Roscioli, Coralie Soulier, Sara Valsecchi, Νikolaos S. Τhomaidis, Emmanuelle Vulliet, Robert B. Young, Saer Samanipour

Bibliographic record

VenueScientific Data · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicIsotope Analysis in Ecology
Canadian institutionsnot available
FundersRijkswaterstaatRECETOX Přírodovědecké Fakulty Masarykovy UniverzityMasarykova UniverzitaCentre National de la Recherche ScientifiqueVlaamse Instelling voor Technologisch OnderzoekUniversitat de GironaÖrebro UniversitetConsiglio Nazionale delle RicercheUniversité Claude Bernard Lyon 1Eidgenössische Anstalt für Wasserversorgung Abwasserreinigung und GewässerschutzUniversität für Bodenkultur WienBureau de Recherches Géologiques et MinièresNational and Kapodistrian University of AthensEuskal Herriko UnibertsitateaSveriges LantbruksuniversitetAarhus Universitets ForskningsfondUniversity of QueenslandVrije Universiteit AmsterdamInstitut National de Recherche pour l'Agriculture, l'Alimentation et l'EnvironnementNorsk Institutt for VannforskningJihočeská Univerzita v Českých BudějovicíchUniversiteit van AmsterdamAgence Nationale de la RechercheAarhus UniversitetCanadian Institute for Advanced ResearchMinistry of Infrastructure and Water ManagementColorado State University
KeywordsSampling (signal processing)Mass spectrometryEnvironmental sciencePassive samplingEnvironmental chemistryChemistryComputer scienceChromatographyStatisticsMathematicsCalibration

Abstract

fetched live from OpenAlex

Non-target analysis (NTA) employing high-resolution mass spectrometry is a commonly applied approach for the detection of novel chemicals of emerging concern in complex environmental samples. NTA typically results in large and information-rich datasets that require computer aided (ideally automated) strategies for their processing and interpretation. Such strategies do however raise the challenge of reproducibility between and within different processing workflows. An effective strategy to mitigate such problems is the implementation of inter-laboratory studies (ILS) with the aim to evaluate different workflows and agree on harmonized/standardized quality control procedures. Here we present the data generated during such an ILS. This study was organized through the Norman Network and included 21 participants from 11 countries. A set of samples based on the passive sampling of drinking water pre and post treatment was shipped to all the participating laboratories for analysis, using one pre-defined method and one locally (i.e. in-house) developed method. The data generated represents a valuable resource (i.e. benchmark) for future developments of algorithms and workflows for NTA experiments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.597
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0020.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0080.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.283
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2021
Admission routes1
Has abstractyes

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