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Record W3204016944 · doi:10.15278/isms.2021.wi03

DETERMINATION OF THE IONIZATION ENERGY OF THE METASTABLE 2 <sup>1</sup>S<sub>0</sub> STATE OF <sup>4</sup>He THROUGH RYDBERG-SERIES EXTRAPOLATION

2021· article· en· W3204016944 on OpenAlexaboutno aff
Gloria Clausen, F. Merkt, Hansjürg Schmutz, Josef A. Agner, Paul Jansen

Bibliographic record

VenueProceedings of the 2021 International Symposium on Molecular Spectroscopy · 2021
Typearticle
Languageen
FieldPhysics and Astronomy
TopicQuantum, superfluid, helium dynamics
Canadian institutionsnot available
Fundersnot available
KeywordsMetastabilityIonizationAtomic physicsState (computer science)PhysicsEnergy (signal processing)ChemistryAnalytical Chemistry (journal)IonMathematics

Abstract

fetched live from OpenAlex

\\noindent Helium, as one of the simplest few-electron atoms, is well suited to test fundamental interactions and QED calculations with a high precision. Its importance is underlined by recent advances in the determination of particle properties such as the $\\alpha$-particle charge radius\\footnote{J. Krauth et al., Nature 589, 527531 (2021)}. Yet, the most accurate theoretical\\footnote{K. Pachucki, V. Patk\\'o$\\check{\\mathrm{s}}$, and V. A. Yerokhin, Physical Review A 95, 062510 (2017)}$^,$\\footnote{G. W. Drake and Z. C. Yan, Canadian Journal of Physics 86, 45 (2008)}\n%\\footnote{ V. Patk\\'o$\\check{\\mathrm{s}}$, V. A. Yerokhin, and K. Pachucki, Physical Review A 103, 012803 (2021)}$^,$\nand experimental\\footnote{W. Lichten, D. Shiner, and Z.-X. Zhou, Physical Review A 43, 1663 (1991)}$^,$\\footnote{C. J. Sansonetti and J. D. Gillaspy, Physical Review A 45, R1 (1992)} data on the ionization energies of the low-lying electronic states show a significant discrepancy of more than 2 $\\sigma$ (about 3 MHz). We report on the determination of the ionization energy of the metastable 2 $^1\\mathrm{S}_0$ state of helium through Rydberg-series extrapolation with a relative uncertainty of $5 \\times 10^{-11}$ through the determination of 20 different $n\\mathrm{p} \\leftarrow2\\;^1\\mathrm{S}_0$ transition frequencies in the range of $n$ from 24 to 102, yielding quantum-defect parameters for the $n$p Rydberg states. A one-photon excitation scheme was employed, using the frequency-doubled output of a narrowband cw laser source (312 nm), calibrated to a frequency comb referenced to a GPS-disciplined Rb clock. The major sources of systematic uncertainties are minimized by (i) carrying out the experiment in a doubly skimmed, pulsed supersonic beam of metastable $^4$He atoms to minimize the Doppler broadening, (ii) compensating electric stray fields to below 0.7 mV/cm, and (iii) cancelling the first-order Doppler shift by monitoring two Doppler components resulting from two counter-propagating laser beams. The effects of residual stray electric fields are included as DC-Stark shifts in the analysis. Our new value of the ionization energy of the $2\\;^1\\mathrm{S}_0$ state of $^4$He, with an absolute uncertainty better than 50 kHz, represents an improvement by a factor of about five in precision. It also allows for a purely experimental determination of the ionization energies of several other low-lying electronic states of $^4$He, which were previously only accurately known through combination of measured and theoretical energy intervals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.143
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.002
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0020.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.219
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2021
Admission routes1
Has abstractyes

Explore more

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