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Record W3208047788 · doi:10.1021/acs.iecr.1c03000

Deposition of Fine Particles during Hydrotreating of Oil Sands Bitumen-Derived Heavy Gas Oil in a Packed Bed Reactor: Impact of Process Parameters and Surface Charge

2021· article· en· W3208047788 on OpenAlexafffund
John Eleeza, V. Sundaramurthy, Philip Boahene, Ajay K. Dalai, John Adjaye

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2021
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsSyncrude (Canada)University of Saskatchewan
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsSyncrude
KeywordsHydrodesulfurizationDeposition (geology)Oil sandsSpace velocityPacked bedTrickle-bed reactorChemistryAsphalteneCatalysisFuel oilChemical engineeringAsphaltMaterials scienceWaste managementComposite materialChromatographySedimentOrganic chemistryGeology

Abstract

fetched live from OpenAlex

Heavy gas oil feed in a packed bed reactor was used to study the influence of temperature (370–400 °C), pressure (1000–1400 psig), and liquid hourly space velocity (LHSV) (0.5–2 h –1 ) on the deposition of fines (asphaltene-coated kaolin) during hydrotreating. The effects of surface charge on fines deposition on the catalyst bed were also investigated. The study showed that LHSV was the only factor with an individual effect on deposition, where increasing LHSV resulted in a decrease in fines deposition. Contrastingly, pressure and temperature showed interactive effects with a combination of high temperature (>380 °C) and low pressure (<1250 psig) or low temperature (<390 °C) and high pressure (>1150 psig), resulting in minimal deposition. These combinations of temperature and pressure also coincided with the region of high hydrodesulfurization, suggesting the impact of fines deposition on catalyst activity. Opposite surface charges possessed by fines and the catalyst created an attractive force that contributed to fines deposition during hydrotreating.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.996
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.043
GPT teacher head0.316
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2021
Admission routes2
Has abstractyes

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