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Record W3210973319 · doi:10.1111/maps.13750

Heating of carbonaceous materials: Insights into the effects of thermal metamorphism on spectral properties of carbonaceous chondrites and asteroids

2021· article· en· W3210973319 on OpenAlexaff
A. C. Duan, Yunzhao Wu, E. A. Cloutis, Jinfei Yu, Shaolin Li, Yun Jiang

Bibliographic record

VenueMeteoritics and Planetary Science · 2021
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAstro and Planetary Science
Canadian institutionsUniversity of Winnipeg
Fundersnot available
KeywordsChondriteMeteoriteMurchison meteoriteAsteroidAbsorption (acoustics)Carbon fibersCarbonaceous chondriteAstrobiologyChemistryParent bodyAbsorption spectroscopySpectral lineEarth (classical element)AnthraciteCoalMineralogyAnalytical Chemistry (journal)Materials scienceOrganic chemistryPhysicsOptics

Abstract

fetched live from OpenAlex

Abstract Carbonaceous chondrites (CCs) are important materials for understanding the early evolution of the solar system and delivery of organic material to the early Earth. Spectral analysis of CCs can establish the relationship between them and their possible parent asteroids, which helps to determine the surface composition of the asteroid. In this paper, the 0.3–26 μm reflectance spectra of a series of coals ranging from lignite to anthracite (Earth analogs of organic matter contained in CCs), a coal heated to various durations and temperatures, and reflectance spectra of CM2 meteorites were analyzed in conjunction with compositional information to derive spectral–compositional relationships. All types of coals have strong aromatic absorptions (3.28 and 5–6.5 μm) and aliphatic “triplet” absorptions (3.38, 3.41, and 3.48 μm). In contrast, CM2 meteorites have obvious aliphatic absorptions and lack aromatic absorptions. The reason is the weak absorption coefficients of aromatic materials and the overlap with strong OH/H 2 O absorption. Absorptions in the coal spectra are strongly related to elemental H/C ratio. When the H/C ratio is >0.55, the absorption intensity of an aliphatic increases linearly with the increase of H/C. For heated coal, increasing heating time above 1 h at 450 °C causes the disappearance of the aliphatic “triplet” absorptions. Similarly, heating Murchison meteorite to 400 °C for 1 week causes all the organic absorptions to disappear. This implies that in remote sensing detections, only asteroids (e.g., with CM and CI carbonaceous chondrites compositions) that experienced low thermal metamorphism (<400 °C) are suitable as potential targets for detecting organic compounds using features in the 3–4 µm region.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.045
Threshold uncertainty score0.395

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.183
Teacher spread0.177 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2021
Admission routes1
Has abstractyes

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