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Record W3212432462 · doi:10.48550/arxiv.2108.13218

Bio-inspired adaptive sensing through electropolymerization of organic\n electrochemical transistors

2021· article· en· W3212432462 on OpenAlexaff
Mahdi Ghazal, Michel Daher Mansour, Corentin Scholaert, Thomas Dargent, Yannick Coffinier, Sébastien Pecqueur, Fabien Alibart

Bibliographic record

VenuearXiv (Cornell University) · 2021
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsInstitut interdisciplinaire d'innovation technologiqueUniversité de Sherbrooke
FundersEuropean Research Council
KeywordsMaterials sciencePEDOT:PSSTransconductanceNanotechnologyTransistorDielectric spectroscopyCapacitanceOptoelectronicsRaman spectroscopyMicrofabricationPolystyrene sulfonateElectrochemistryElectrodeVoltageLayer (electronics)Electrical engineering

Abstract

fetched live from OpenAlex

Organic Electrochemical Transistors are considered today as a key technology\nto interact with biological medium through their intrinsic ionic-electronic\ncoupling. In this paper, we show how this coupling can be finely tuned (in\noperando) post-microfabrication via electropolymerization technique. This\nstrategy exploits the concept of adaptive sensing where both transconductance\nand impedance are tunable and can be modified on-demand to match different\nsensing requirements. Material investigation through Raman spectroscopy, atomic\nforce microscopy and scanning electron microscopy reveals that\nelectropolymerization can lead to a fine control of PEDOT microdomains\norganization, which directly affect the iono-electronic properties of OECTs. We\nfurther highlight how volumetric capacitance and effective mobility of\nPEDOT:PSS influence distinctively the transconductance and impedance of OECTs.\nThis approach shows to improve the transconductance by 150% while reducing\ntheir variability by 60% in comparison with standard spin-coated OECTs.\nFinally, we show how to the technique can influence voltage spike rate hardware\nclassificationwith direct interest in bio-signals sorting applications.\n

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.155
Threshold uncertainty score0.520

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.043
GPT teacher head0.183
Teacher spread0.140 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2021
Admission routes1
Has abstractyes

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