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Understanding the Properties of Bitumen Froth from Oil Sands Surface Mining and Treatment of Water-in-Oil Emulsions

2021· article· en· W3216208541 on OpenAlexafffundabout
Duo Wang, Chenyu Qiao, Ziqian Zhao, Wenshuai Yang, Hongyun Chen, Taiheng Yin, Zhiling Yan, Meng Wu, Xiaohui Mao, Camila Santander, Qi Liu, Qingxia Liu, Petr A. Nikrityuk, Tian Tang, Hongbo Zeng

Bibliographic record

VenueEnergy & Fuels · 2021
Typearticle
Languageen
FieldEngineering
TopicEnhanced Oil Recovery Techniques
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanada Foundation for Innovation
KeywordsAsphaltOil sandsWettingContact angleAdsorptionChemical engineeringAsphalteneEnergy-dispersive X-ray spectroscopyScanning electron microscopeX-ray photoelectron spectroscopyTolueneMaterials scienceEmulsionChemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Bitumen froth, as the crude product from the surface mining of oil sands, requires the efficient removal of water and solids for further processing. This work has systematically characterized the properties of bitumen froth from an oil sands operation in Northern Alberta and their correlation to the froth treatment efficiency (i.e., removal of water and demulsification behaviors). Systematic characterization was performed regarding the composition, wettability, and particle size distribution of the solids separated from different phases (i.e., diluted bitumen, aqueous phase, and coarse solids). Multiscale analyses including X-ray photoelectron spectroscopy (XPS), scanning electron microscopy coupled with energy dispersive X-ray spectroscopy (SEM/EDX), X-ray powder diffraction (XRD), and elemental analysis were employed to analyze the surface and bulk chemistry of the solids. The results indicate that a great amount of toluene-soluble and toluene-insoluble organics are discontinuously adsorbed on the solid surfaces, making the solid biwettable with a water contact angle of around 90°. The biwettable and fine solids are apt to remain at the oil/water interface or are trapped between the oil droplets, strengthening the “protective” interfacial film, which contributes to the formation of rag layer. The fine and ultrafine solids with a surface coating of organics remain with bitumen and adversely influence the quality of the separated bitumen. The organic-coated coarse solids precipitate toward the bottom, reducing the overall bitumen recovery. In addition, a trace amount of the organics could be firmly adsorbed on the solid surface, which further impedes the demulsification efficiency. This work correlates the characteristics of the bitumen froth and its demulsification efficiency using two commercial demulsifiers, with useful implications for developing effective and cost-efficient demulsifiers and emulsion treatment technologies in oil production and other related chemical and engineering processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.039
Threshold uncertainty score0.078

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.215
Teacher spread0.175 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2021
Admission routes3
Has abstractyes

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