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Record W3217437752 · doi:10.1063/5.0075412

Computing vibrational energy levels by solving linear equations using a tensor method with an imposed rank

2021· article· en· W3217437752 on OpenAlex
Sangeeth Das Kallullathil, Tucker Carrington

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Journal of Chemical Physics · 2021
Typearticle
Languageen
FieldMathematics
TopicTensor decomposition and applications
Canadian institutionsQueen's University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsRank (graph theory)Tensor (intrinsic definition)Basis (linear algebra)OrthogonalizationApplied mathematicsMathematicsBasis functionHamiltonian (control theory)Realization (probability)Tensor productAlgorithmMathematical analysisMathematical optimizationPure mathematicsCombinatoricsGeometry

Abstract

fetched live from OpenAlex

Present day computers do not have enough memory to store the high-dimensional tensors required when using a direct product basis to compute vibrational energy levels of a polyatomic molecule with more than about five atoms. One way to deal with this problem is to represent tensors using a tensor format. In this paper, we use the canonical polyadic (CP) format. Energy levels are computed by building a basis from vectors obtained by solving linear equations. The method can be thought of as a CP realization of a block inverse iteration method with multiple shifts. The CP rank of the tensors is fixed, and the linear equations are solved with an method. There is no need for rank reduction and no need for orthogonalization, and tensors with a rank larger than the fixed rank used to solve the linear equations are never generated. The ideas are tested by computing vibrational energy levels of a 64-D bilinearly coupled model Hamiltonian and of acetonitrile (12-D).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.422
Threshold uncertainty score0.331

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.078
GPT teacher head0.360
Teacher spread0.282 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it