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Record W3217676370 · doi:10.1002/aenm.202102556

Advanced Support Materials and Interactions for Atomically Dispersed Noble‐Metal Catalysts: From Support Effects to Design Strategies

2021· article· en· W3217676370 on OpenAlex
Xu‐Lei Sui, Lei Zhang, Junjie Li, Kieran Doyle‐Davis, Ruying Li, Zhen‐Bo Wang, Xueliang Sun

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Energy Materials · 2021
Typearticle
Languageen
FieldEnergy
TopicElectrocatalysts for Energy Conversion
Canadian institutionsWestern University
FundersChina Scholarship CouncilWestern UniversityNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaCanada Research Chairs
KeywordsNoble metalMaterials scienceNanotechnologyCatalysisMechanism (biology)MetalChemistryMetallurgy

Abstract

fetched live from OpenAlex

Abstract Indisputably, noble‐metal single atom catalysts (SACs) are one of the most popular research topics in the field of catalysis because of their low cost, ultrahigh atomic utilization, and distinctive performance for a wide variety of catalytic reactions. Support materials play a vital role in the preparation and catalytic performance of noble‐metal SACs. Thus, diverse support materials have been developed very rapidly and elaborately designed in the last few years. In this review, the support effects in noble‐metal SACs are first systematically introduced, including anchoring effects, strong metal–support interactions, and synergistic catalysis effects. Moreover, the most recent advances in support materials are classified and discussed in detail with a focus on their anchoring mechanism. Importantly, design strategies for advanced supports are summarized for guiding the development and utilization of advanced support materials. To conclude possible future research directions for support materials are put forward to help overcome the current issues facing noble‐metal SACs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.036
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.250
Teacher spread0.241 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it