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Record W4200560887 · doi:10.1002/aenm.202102715

Dual‐Metal Atom Electrocatalysts: Theory, Synthesis, Characterization, and Applications

2021· article· en· W4200560887 on OpenAlexfundno aff
Angus Pedersen, Jesús Barrio, Alain Y. Li, Rhodri Jervis, Dan J. L. Brett, Maria‐Magdalena Titirici, Ifan E. L. Stephens

Bibliographic record

VenueAdvanced Energy Materials · 2021
Typearticle
Languageen
FieldEnergy
TopicElectrocatalysts for Energy Conversion
Canadian institutionsnot available
FundersEuropean Research CouncilEngineering and Physical Sciences Research CouncilNational Research Council CanadaEuropean Commission
KeywordsElectrocatalystElectrochemical energy conversionMaterials scienceCommercializationCharacterization (materials science)NanotechnologyElectrochemistryDual (grammatical number)CatalysisSustainable energyAtom (system on chip)Electrochemical energy storageEnergy transformationAtom economyCombinatorial chemistryBiochemical engineeringComputer scienceSupercapacitorPhysical chemistryElectrical engineeringChemistryPhysicsRenewable energyElectrodeEngineeringOrganic chemistryThermodynamicsBusiness

Abstract

fetched live from OpenAlex

Abstract Electrochemical clean energy conversion and the production of sustainable chemicals are critical in the journey to realizing a truly sustainable society. To progress electrochemical storage and conversion devices to commercialization, improving the electrocatalyst performance and cost are of utmost importance. Research into dual‐metal atom catalysts (DACs) is rising in prominence due to the advantages of these sites over single‐metal atom catalysts (SACs), such as breaking scaling relationships for the adsorption energy of reaction intermediates and synergistic effects. This review provides an examination of the fundamental theoretical principles and experimental electrochemical performance of DACs in idealized half cells, as well as fuel cells, before proceeding to analyze the methods used for producing and identifying DACs. Current challenges and potential future research directions of DACs are also discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.331
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.205
Teacher spread0.201 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations174
Published2021
Admission routes1
Has abstractyes

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