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Record W4206805786 · doi:10.1063/5.0064517

High-field magnetic resonance imaging: Challenges, advantages, and opportunities for novel contrast agents

2022· article· en· W4206805786 on OpenAlexafffund
Abhinandan Banerjee, Barbara Błasiak, Armita Dash, Bogusław Tomanek, Frank C. J. M. van Veggel, Simon Trudel

Bibliographic record

VenueChemical Physics Reviews · 2022
Typearticle
Languageen
FieldMaterials Science
TopicLanthanide and Transition Metal Complexes
Canadian institutionsUniversity of VictoriaUniversity of CalgaryUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaAlberta Innovates - Health SolutionsUniversity of Calgary
KeywordsContrast (vision)Magnetic resonance imagingComputer scienceModalitiesField (mathematics)High contrastNuclear magnetic resonanceMaterials scienceMedical physicsNanotechnologyArtificial intelligenceRadiologyMedicinePhysicsOpticsMathematics

Abstract

fetched live from OpenAlex

There is a need for non-invasive diagnostic tools to detect and monitor the occurrence of diseases. Ideally, this can be done without resorting to ionizing radiation, especially when multiple rounds of imaging are required. Magnetic resonance imaging (MRI), a form of three-dimensional nuclear magnetic resonance, has become a common tool of choice for diagnosticians. Due to the low contrast difference between healthy and diseased tissue, contrast agents—magnetic species administered to the patient prior to imaging—are routinely used for contrast improvement. High-field (B0 ≥ 4.7 T, 1H Larmor frequency ≥ 200 MHz) MRI offers advantages in terms of better signal-to-noise ratio, as well as improved spectral resolution for certain applications. New contrast agents are being developed for high-field MRI, the topic of this review. After discussing the purpose of contrast agents and the advantages and potential issues of high-field MRI, we discuss recent developments in the field of contrast agent design, synthesis, and applications, citing examples of high-field MRI-ready molecular contrast agents, as well as nanoparticulate contrast agents based on various inorganic materials (e.g., coordination polymers, transition metal oxides, or lanthanide halides). We will discuss how certain aspects (composition, shape, ligands) affect the contrasting abilities of these agents. Finally, we highlight recent developments in the promising field of multifunctional probes, wherein multiple imaging and/or therapeutic modalities are combined in a single species. As high-field MRI becomes more commonplace in the clinical setting, such new contrast agents are needed to provide optimized imaging. This will facilitate the clinician's task in resolving pathologies for more efficient diagnosis and patient treatment.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.833
Threshold uncertainty score0.550

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.117
GPT teacher head0.295
Teacher spread0.178 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2022
Admission routes2
Has abstractyes

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