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Record W4210653458 · doi:10.1016/j.cej.2022.135058

Biowaste-derived electrode and electrolyte materials for flexible supercapacitors

2022· article· en· W4210653458 on OpenAlex
Yazan Al Haj, Seyedabolfazl Mousavihashemi, Daria Robertson, Maryam Borghei, Timo Pääkkönen, Orlando J. Rojas, Eero Kontturi, Tanja Kallio, Jaana Vapaavuori

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemical Engineering Journal · 2022
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsUniversity of British Columbia
FundersBusiness FinlandProject 211Magnus Ehrnroothin SäätiöAalto-YliopistoEuropean Commission
KeywordsSupercapacitorElectrolyteMaterials scienceCapacitanceElectrodePower densityEnergy storageChemical engineeringElectrochemistrySeparator (oil production)Composite materialNanotechnologyChemistryPower (physics)

Abstract

fetched live from OpenAlex

One of the key challenges in the development of energy storage devices relates to material sourcing in harmony with clean technologies. Herein, cellulose nanocrystals (CNC) extracted from brewery residues are used as transparent hydrogel electrolyte after physical cross-linking with aluminum ions (Al3+). The hydrogel electrolyte (Al-CNC) exhibits an ultrahigh ionic conductivity (∼24.9 mS cm−1), high optical transmittance (∼92.9% at 550 nm wavelength), outstanding compression strength (3.9 MPa at a 70% strain), and tolerates to various deformations (e.g., twisting, folding, rolling). Meanwhile, animal bone biowaste is used to synthesize porous carbon (PC) electrodes (∼879 m2 g−1) that are effective in delivering an outstanding specific capacitance (∼804 F g−1 at 1 A g−1). A fully renewable flexible symmetric supercapacitor is assembled by sandwiching the Al-CNC hydrogel between two bone-derived PC electrodes (PC//Al-CNC//PC). The obtained flexible device displays a high energy density (18.2 Wh kg−1 at 1 425 W kg−1), exceptional power density (20 833 W kg−1 at 7.1 Wh kg−1), and ∼92% capacitance retention after 6 000 cycles at 5 A g−1. We further demonstrated the biowaste-derived high-performance flexible supercapacitors for their mechanical durability and reliable electrochemical performance under bending cycles. All combined, the devices are shown to be ideally suited for renewable energy storage applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.705

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.205
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it