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Record W4210821159 · doi:10.1038/s42005-022-00805-6

Correlation-driven electronic reconstruction in FeTe1−xSex

2022· article· en· W4210821159 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueCommunications Physics · 2022
Typearticle
Languageen
FieldMaterials Science
TopicIron-based superconductors research
Canadian institutionsCanadian Light Source (Canada)University of British Columbia
FundersDivision of Materials Sciences and EngineeringLawrence Berkeley National LaboratoryNational Science FoundationLaboratory Directed Research and DevelopmentNational Key Research and Development Program of ChinaGordon and Betty Moore FoundationMaterials Research Science and Engineering Center, Harvard UniversityCanada First Research Excellence FundOffice of ScienceRice UniversityUniversity of TokyoRenmin University of ChinaNational Nuclear Security AdministrationSun Yat-sen UniversityU.S. Department of EnergyNational Natural Science Foundation of ChinaDivision of Materials ResearchUniversity of SaskatchewanBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaLos Alamos National LaboratoryUniversity of WashingtonAlfred P. Sloan FoundationCanadian Light SourceCanadian Institutes of Health ResearchWelch Foundation
KeywordsChalcogenideElectronic correlationCondensed matter physicsAtomic orbitalSuperconductivityPhase diagramCuprateElectronic structurePhase (matter)Fermi surfacePhysicsMaterials scienceElectronQuantum mechanics

Abstract

fetched live from OpenAlex

Abstract Electronic correlation is of fundamental importance to high temperature superconductivity. While the low energy electronic states in cuprates are dominantly affected by correlation effects across the phase diagram, observation of correlation-driven changes in fermiology amongst the iron-based superconductors remains rare. Here we present experimental evidence for a correlation-driven reconstruction of the Fermi surface tuned independently by two orthogonal axes of temperature and Se/Te ratio in the iron chalcogenide family FeTe 1− x Se x . We demonstrate that this reconstruction is driven by the de-hybridization of a strongly renormalized d x y orbital with the remaining itinerant iron 3 d orbitals in the emergence of an orbital-selective Mott phase. Our observations are further supported by our theoretical calculations to be salient spectroscopic signatures of such a non-thermal evolution from a strongly correlated metallic phase into an orbital-selective Mott phase in d x y as Se concentration is reduced.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.641
Threshold uncertainty score0.977

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.301
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it