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Record W4213361005 · doi:10.1029/2021jd035570

High Resolution Dynamical Analysis of Volatile Organic Compounds (VOC) Measurements During the BIO‐MAÏDO Field Campaign (Réunion Island, Indian Ocean)

2022· article· en· W4213361005 on OpenAlexaff
Manon Rocco, Jean‐Luc Baray, Aurélie Colomb, Agnès Borbon, Pamela Dominutti, Pierre Tulet, Crist Amelynck, Niels Schoon, Bert Verreyken, Valentin Duflot, Valérie Gros, Roland Sarda‐Estève, Guillaume Péris, Christian Guadagno, Maud Leriche

Bibliographic record

VenueJournal of Geophysical Research Atmospheres · 2022
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsUniversité du Québec à Montréal
FundersBelgian Federal Science Policy OfficeAgence Nationale de la Recherche
KeywordsIsopreneEnvironmental scienceAtmospheric sciencesVolatile organic compoundAdvectionChemistryMeteorologyEnvironmental chemistryGeographyPhysicsThermodynamics

Abstract

fetched live from OpenAlex

Abstract This study presents a high‐resolution dynamical analysis of Volatile Organic Compound (VOC) concentrations measured from March 11 to April 4 2019 at Réunion Island during the BIO‐MAÏDO (Bio‐physicochemistry of tropical clouds at Maïdo: processes and impacts on secondary organic aerosols formation) campaign. We detail the dynamical and chemical processes that govern atmospheric VOC concentrations at two targeted sites of the western slope of Réunion Island: Petite France (PF), 950 m above sea level (a.s.l.) and Maïdo Observatory (MO), 2150 m a.s.l. A dynamical connection between PF and MO is found during four selected days: March 28 and 31, April 1 and 3. Trajectory calculations using the coupling of Meso‐Computing Advection‐interpolation of atmospheric parameters and Trajectory tool (CAT) (100 m horizontal resolution of Meso‐NH high‐resolution non‐hydrostatic model and the CAT trajectory model) Lagrangian transport model showed that air masses were dynamically linked between the two measurements sites for 44.8% of the time during the complete campaign. Trajectories from the Meso‐CAT model combined with the Corine Land Cover‐2018 register shows that backward‐trajectories are frequently located above biogenic area (mixed forest, 8%–67% of total number trajectory point) and cultures area (e.g., sugar cane plantation, 0%–21%). Regarding VOCs concentrations, air masses coming from downhill MO are associated with significant measured concentrations of isoprene, isoprene oxidation products and benzene. Averaged concentration daytime ratios of isoprene and isoprene oxidation products from PF to MO are 0.73 ± 1.01 and 0.26 ± 0.26 respectively illustrating a loss of these VOCs due to deposition, oxidation, or possibility dilution on clouds.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.151
Threshold uncertainty score0.301

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.262
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations22
Published2022
Admission routes1
Has abstractyes

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