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Record W4214670654 · doi:10.1038/s41563-022-01203-7

Superconductivity in (Ba,K)SbO3

2022· article· en· W4214670654 on OpenAlexafffund
Minu Kim, Graham McNally, Hun-ho Kim, Mohamed Oudah, Alexandra S. Gibbs, Pascal Manuel, Robert J. Green, Ronny Sutarto, T. Takayama, A. N. Yaresko, Ulrich Wedig, Masahiko Isobe, Reinhard K. Kremer, D. A. Bonn, B. Keimer, H. Takagi

Bibliographic record

VenueNature Materials · 2022
Typearticle
Languageen
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsUniversity of SaskatchewanCanadian Light Source (Canada)University of British Columbia
FundersEngineering and Physical Sciences Research CouncilCanadian Institutes of Health ResearchUniversity of British ColumbiaScience and Technology Facilities CouncilUniversity of TokyoResearch Councils UKMax-Planck-GesellschaftUniversity of SaskatchewanCanadian Light Source
KeywordsSuperconductivityCharge density waveCondensed matter physicsCharge (physics)Charge densityMaterials scienceDensity of statesMetalBand gapChemistryPhysics

Abstract

fetched live from OpenAlex

Abstract (Ba,K)BiO 3 constitute an interesting class of superconductors, where the remarkably high superconducting transition temperature T c of 30 K arises in proximity to charge density wave order. However, the precise mechanism behind these phases remains unclear. Here, enabled by high-pressure synthesis, we report superconductivity in (Ba,K)SbO 3 with a positive oxygen–metal charge transfer energy in contrast to (Ba,K)BiO 3 . The parent compound BaSbO 3− δ shows a larger charge density wave gap compared to BaBiO 3 . As the charge density wave order is suppressed via potassium substitution up to 65%, superconductivity emerges, rising up to T c = 15 K. This value is lower than the maximum T c of (Ba,K)BiO 3 , but higher by more than a factor of two at comparable potassium concentrations. The discovery of an enhanced charge density wave gap and superconductivity in (Ba,K)SbO 3 indicates that strong oxygen–metal covalency may be more essential than the sign of the charge transfer energy in the main-group perovskite superconductors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.072
Threshold uncertainty score0.928

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0730.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.208
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations74
Published2022
Admission routes2
Has abstractyes

Explore more

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