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Record W4214888571 · doi:10.3390/molecules27051659

Application of Rhamnolipids as Dispersing Agents for the Fabrication of Composite MnO2-Carbon Nanotube Electrodes for Supercapacitors

2022· article· en· W4214888571 on OpenAlexafffund
Wenjuan Yang, Wenyu Liang, Igor Zhitomirsky

Bibliographic record

VenueMolecules · 2022
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsMcMaster University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSupercapacitorMaterials scienceCapacitanceElectrodeFabricationCarbon nanotubeNanocompositeCyclic voltammetryNanotechnologyComposite numberDispersantChemical engineeringDispersion (optics)Composite materialElectrochemistryChemistry

Abstract

fetched live from OpenAlex

The high theoretical capacitance of MnO2 renders it a promising material for the cathodes of asymmetric supercapacitors. The good dispersion of MnO2 and conductive additives in a nanocomposite electrode is a key factor for efficient electrode performance. This article describes, for the first time, the application of rhamnolipids (RL) as efficient natural biosurfactants for the fabrication of nanocomposite MnO2-carbon nanotube electrodes for supercapacitors. RL act as co-dispersants for MnO2 and carbon nanotubes and facilitate their efficient mixing, which allows for advanced capacitive properties at an active mass of 40 mg cm−2 in Na2SO4 electrolytes. The highest capacitance obtained from the cyclic voltammetry data at a scan rate of 2 mV s−1 is 8.10 F cm−2 (202.6 F g−1). The highest capacitance obtained from the galvanostatic charge–discharge data at a current density of 3 mA cm−2 is 8.65 F cm−2 (216.16 F g−1). The obtained capacitances are higher than the capacitances of MnO2-based electrodes of the same active mass reported in the literature. The approach developed in this investigation is simple compared to other techniques used for the fabrication of electrodes with high active mass. It offers advantages of using a biocompatible RL biosurfactant.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.252
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2022
Admission routes2
Has abstractyes

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