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Record W4220804494 · doi:10.5194/bg-19-359-2022

Ideas and perspectives: Emerging contours of a dynamic exogenous kerogen cycle

2022· article· en· W4220804494 on OpenAlexaboutno aff
Thomas M. Blattmann

Bibliographic record

VenueBiogeosciences · 2022
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeology and Paleoclimatology Research
Canadian institutionsnot available
FundersJapan Agency for Marine-Earth Science and Technology
KeywordsKerogenWeatheringGlacial periodGeologyEarth scienceDeglaciationCarbon cycleIce coreSnowball EarthIsotopes of carbonPaleontologyOceanographyTotal organic carbonSource rockChemistryEnvironmental chemistryEcology

Abstract

fetched live from OpenAlex

Abstract. Growing evidence points to the dynamic role that kerogen is playing on Earth's surface in controlling atmospheric chemistry over geologic time. Although quantitative constraints on the weathering of kerogen remain loose, its changing weathering behavior modulated by the activity of glaciers suggests that this largest pool of reduced carbon on Earth may have played a key part in atmospheric CO2 variability across recent glacial–interglacial cycles and beyond. This work enunciates the possibility of kerogen oxidation as a major driver of atmospheric CO2 increase in the wake of glacial episodes. This hypothesis of centennial- and millennial-timescale relevance for this chemical weathering pathway is substantiated by several lines of independent evidence synthesized in this contribution, including the timing of atmospheric CO2 increase, atmospheric CO2 isotope composition (13C and 14C), kerogen oxidation kinetics, observations of kerogen reburial, and modeling results. The author hypothesizes that the deglaciation of kerogen-rich lithologies in western Canada contributed to the characteristic deglacial increase in atmospheric CO2, which reached an inflection point ≤ 300 years after the Laurentide Ice Sheet retreated into the kerogen-poor Canadian Shield. To reconcile the release of isotopically light carbon via kerogen oxidation with Earth surface carbon pool constraints, major oceanic degassing and biospheric regrowth must have acted in concert across glacial–interglacial transitions. Additionally, a process such as a strong shift in the ratio of C3 to C4-derived organic matter must be invoked to maintain isotope mass balance, a point key for reconciling the hypothesis with the carbon isotope record of marine dissolved inorganic carbon. In order to test this hypothesis, quantitative constraints on the contribution of kerogen oxidation to CO2 rise at glacial terminations are needed through systematic studies on (1) CO2 fluxes emanating from the weathering of different lithologies, (2) oxidation kinetics of kerogen along glacial chronosequences, and (3) high-resolution temporal changes in the aerial extent of glacially exposed lithological units and glacial flour.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.024
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.249
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2022
Admission routes1
Has abstractyes

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