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Record W4220892682 · doi:10.3390/catal12030324

Formic Acid Dehydrogenation Using Noble-Metal Nanoheterogeneous Catalysts: Towards Sustainable Hydrogen-Based Energy

2022· article· en· W4220892682 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueCatalysts · 2022
Typearticle
Languageen
FieldChemical Engineering
TopicCarbon dioxide utilization in catalysis
Canadian institutionsMemorial University of Newfoundland
FundersUniversity Of Al-QadisiyahMemorial University of Newfoundland
KeywordsDehydrogenationFormic acidCatalysisHydrogen storageHydrogenBimetallic stripHydrogen fuelCarbon monoxideNoble metalInorganic chemistryMaterials scienceChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

The need for sustainable energy sources is now more urgent than ever, and hydrogen is significant in the future of energy. However, several obstacles remain in the way of widespread hydrogen use, most of which are related to transport and storage. Dilute formic acid (FA) is recognized asa a safe fuel for low-temperature fuel cells. This review examines FA as a potential hydrogen storage molecule that can be dehydrogenated to yield highly pure hydrogen (H2) and carbon dioxide (CO2) with very little carbon monoxide (CO) gas produced via nanoheterogeneous catalysts. It also present the use of Au and Pd as nanoheterogeneous catalysts for formic acid liquid phase decomposition, focusing on the influence of noble metals in monometallic, bimetallic, and trimetallic compositions on the catalytic dehydrogenation of FA under mild temperatures (20–50 °C). The review shows that FA production from CO2 without a base by direct catalytic carbon dioxide hydrogenation is far more sustainable than existing techniques. Finally, using FA as an energy carrier to selectively release hydrogen for fuel cell power generation appears to be a potential technique.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.030
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.002
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.227
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it