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Record W4221014622 · doi:10.1002/adma.202110585

Bioinspired Tough Solid‐State Electrolyte for Flexible Ultralong‐Life Zinc–Air Battery

2022· article· en· W4221014622 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Materials · 2022
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsUniversity of Waterloo
FundersGuangdong Science and Technology DepartmentNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsMaterials scienceElectrolyteNanotechnologyConductivityQuasi-solidBattery (electricity)Chemical engineeringElectrodeChemistry

Abstract

fetched live from OpenAlex

Abstract Manufacturing advanced solid‐state electrolytes (SSEs) for flexible rechargeable batteries becomes increasingly important but remains grand challenge. The sophisticated structure of robust animal dermis and good water‐retention of plant cell in nature grant germane inspirations for designing high‐performance SSEs. Herein, tough bioinspired SSEs with intrinsic hydroxide ion (OH − ) conduction are constructed by in situ formation of OH − conductive ionomer network within a hollow‐polymeric‐microcapsule‐decorated hydrogel polymer network. By virtue of the bioinspired design and dynamic dual‐penetrating network structure, the bioinspired SSEs simultaneously obtain mechanical robustness with 1800% stretchability, good water uptake of 107 g g −1 and water retention, and superhigh ion conductivity of 215 mS cm −1 . The nanostructure of bioinspired SSE and related ion‐conduction mechanism are revealed and visualized by molecular dynamics simulation, where plenty of compact and superfast ion‐transport channels are constructed, contributing to superhigh ion conductivity. As a result, the flexible solid‐state zinc–air batteries assembled with bioinspired SSEs witness high power density of 148 mW cm −2 , specific capacity of 758 mAh g −1 and ultralong cycling stability of 320 h as well as outstanding flexibility. The bioinspired methodology and deep insight of ion‐conduction mechanism will shed light on the design of advanced SSEs for flexible energy conversion and storage systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.102
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.271
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it