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Record W4221057920 · doi:10.1080/27658511.2022.2046324

Surface interactions of oxytetracycline on municipal solid waste-derived biochar–montmorillonite composite

2022· article· en· W4221057920 on OpenAlexaff
Madara Weerasooriyagedara, Ahamed Ashiq, Sameera R. Gunatilake, Dimitrios A. Giannakoudakis, Meththika Vithanage

Bibliographic record

VenueSustainable Environment · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsQueen's University
FundersUniversity of Sri Jayewardenepura
KeywordsBiocharAdsorptionComposite numberMontmorilloniteEnvironmental remediationChemical engineeringSpecific surface areaMunicipal solid wasteMaterials scienceFourier transform infrared spectroscopyAqueous solutionChemistryWaste managementNuclear chemistryComposite materialCatalysisOrganic chemistryPyrolysisContamination

Abstract

fetched live from OpenAlex

A composite material prepared from municipal solid waste-derived biochar and montmorillonite (MSW-BC-MMT) was studied as a remediation medium for the removal of oxytetracycline (OTC) from aqueous systems. The morphological characterization using SEM images revealed that the composite had a heterogeneous flaky, plate-like surface appearance. Based on N2 adsorption experiments and compared to the pristine biochar, the composite showed an increased specific surface area by 1.5 folds. The three-parameter Redlich Peterson isotherm model and two-parameter Temkin isotherm model were best fitted with R2 = 0.998 and 0.997, respectively, both for the pristine biochar and the MSW-BC-MMT composite. Additionally, the kinetics was best described using the pseudo-second-order model, suggesting that OTC adsorption onto the composite takes place via chemisorption. A capacity of 233 mg g−1 was observed for the MSW-BC-MMT, which is suggested to be predominantly governed by π-π electron donor–acceptor interactions, electrostatic attraction and surface complexation. As evidenced by FTIR results, OTC was presumed to be adsorbed via hydrogen bonding as well. The value addition of MSW by producing MSW-derived biochar is considered a favorable solution for solid waste management. Therefore, the production of the MSW-BC-MMT composite becomes useful due to its significance in acting as a simultaneous MSW management technique and a low-cost material for antibiotic OTC remediation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.239
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2022
Admission routes1
Has abstractyes

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