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Record W4221070820 · doi:10.3390/w14060987

Removal of Organoselenium from Aqueous Solution by Nanoscale Zerovalent Iron Supported on Granular Activated Carbon

2022· article· en· W4221070820 on OpenAlexafffund
Stanley Onyinye Okonji, Gopal Achari, David Pernitsky

Bibliographic record

VenueWater · 2022
Typearticle
Languageen
FieldEngineering
TopicEnvironmental remediation with nanomaterials
Canadian institutionsStantec (Canada)University of Calgary
FundersPetroleum Technology Development FundNatural Sciences and Engineering Research Council of Canada
KeywordsAdsorptionChemistryZerovalent ironFreundlich equationAqueous solutionNuclear chemistryLangmuir adsorption modelActivated carbonDesorptionWastewaterChromatographyOrganic chemistryWaste management

Abstract

fetched live from OpenAlex

Nanoscale zerovalent iron particles (nZVI) immobilized on coconut shell-based granular activated carbon (GAC) were studied to remove organoselenium from wastewater. A chemical reduction technique that involves the application of sodium borohydride was adopted for the adsorbent preparation. The texture, morphology and chemical composition of the synthesized adsorbents were analyzed with a scanning electron microscope (SEM), nitrogen adsorption–desorption isotherms and X-ray diffraction (XRD). Batch experiment with various pHs and contact times were conducted to evaluate nZVI/GAC adsorption performance. The results showed that nZVI/GAC has a strong affinity to adsorb selenomethionine (SeMet) and selenocysteine (SeCys) from wastewaters. The maximum removal efficiency for the composite (nZVI/GAC) was 99.9% for SeCys and 78.2% for SeMet removal, which was significantly higher than that of nZVI (SeCy, 59.2%; SeMet, 10.8%). The adsorption kinetics were studied by pseudo-first-order (PFO) and pseudo-second-order (PSO) kinetic models. Amongst the two, PSO seemed to have a better fit (SeCy, R2 > 0.998; SeMet, R2 > 0.999). The adsorption process was investigated using Langmuir and Freundlich isotherm models. Electrostatic attraction played a significant role in the removal of organoselenium by nZVI/GAC adsorption. Overall, the results indicated that GAC-supported nZVI can be considered a promising and efficient technology for removing organoselenium from wastewater.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.170
Teacher spread0.165 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2022
Admission routes2
Has abstractyes

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