Anti-Stokes cooling in silica and nanoparticle-doped silicate fibers
Bibliographic record
Abstract
The recent reports of laser cooling in Yb-doped aluminosilicate fibers and silica preforms have opened up the field of optical refrigeration and radiation-balanced lasers to the enormous realm of silica fiber lasers and amplifiers. To increase the cooling efficiency achieved in these materials, it is critical to identify host compositions that improve the Yb<sup>3+</sup>-ion properties in the directions of low concentration quenching, short radiative lifetime, and a long-wavelength absorption tail that extends as far as possible above the zero-phonon line. In this on-going quest, nanoparticle-doped fibers offer a promising technique to modify the chemical environment of the Yb<sup>3+</sup> ions and achieve some of these properties. In this work, three fibers in which the Yb<sup>3+</sup> ions are initially encapsulated in CaF<sub>2,</sub> SrF<sub>2,</sub> or BaF<sub>2 </sub>nanoparticles were fabricated using a solution-doping technique, and their laser-cooling properties evaluated experimentally and analyzed. The CaF<sub>2</sub> fiber and the SrF<sub>2</sub> fiber were successfully cooled at atmospheric pressure when pumped with a continuous-wave laser at the near-optimum wavelength of 1040 nm. The measured maximum temperature change from room temperature was -26.2 mK for the CaF<sub>2</sub> fiber at a pump power absorption level of 90 mW/m, and -16.7 mK at 66 mW/m for the SrF<sub>2</sub> fiber. The BaF<sub>2</sub> fiber did not cool, but it warmed only slightly, indicating that it was not far from cooling. Analysis of the measured dependence of the fiber temperature change on pump power with a model enabled extraction of the fiber’s critical quenching concentration and residual absorptive loss due to impurities. Comparison of these values to the values reported for an aluminosilicate fiber and fiber preforms that cooled shows that the CaF<sub>2</sub> and SrF<sub>2</sub> fibers faired as well as the fiber, and better than the preforms, in terms of quenching, but that they had a higher absorptive loss. This study establishes the significant research potential of nanoparticle-doped fibers in the search for efficient laser-cooling silica hosts.
Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.
How this classification was reachedexpand
Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.001 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.001 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one teacher head, not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".