MétaCan
Menu
Back to cohort
Record W4223622339 · doi:10.1002/chem.202282061

Frontispiece: Electronic Circular Dichroism‐Circularly Polarized Raman (eCP‐Raman): A New Form of Chiral Raman Spectroscopy

2022· paratext· en· W4223622339 on OpenAlexaff
Guojie Li, Mutasem Alshalalfeh, Josef Kapitán, Petr Bouř, Yunjie Xu

Bibliographic record

VenueChemistry - A European Journal · 2022
Typeparatext
Languageen
FieldChemistry
TopicMolecular spectroscopy and chirality
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsRaman spectroscopyRaman optical activityChirality (physics)Vibrational circular dichroismCircular dichroismCoherent anti-Stokes Raman spectroscopyMaterials scienceRaman scatteringExcited stateResolution (logic)Analytical Chemistry (journal)ChemistryMolecular physicsOpticsChiral symmetryCrystallographyAtomic physicsPhysicsOrganic chemistryComputer science

Abstract

fetched live from OpenAlex

A newly developed chiral Raman spectroscopy, eCP-Raman, which combines high chirality sensitivity of electronic CD and high resolution capability of Raman is reported in this Concept article. The model for quantifying eCP-Raman effects is derived and multiple examples, which show strong eCP-Raman responses of solvents and the resonating chiral solutes, are discussed. Its usage in untangling complex excited state phenomena is also mentioned.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.541
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0020.002
Meta-epidemiology (broad)0.0020.002
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0010.000
Open science0.0040.001
Research integrity0.0010.010
Insufficient payload (model declined to judge)0.1190.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.234
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

Explore more

Same venueChemistry - A European JournalSame topicMolecular spectroscopy and chiralityFrench-language works237,207