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Record W4225080063 · doi:10.1103/physrevx.12.011013

Ultrafast Renormalization of the On-Site Coulomb Repulsion in a Cuprate Superconductor

2022· article· en· W4225080063 on OpenAlex
Denitsa Baykusheva, Hoyoung Jang, Ali Husain, Sangjun Lee, Sophia F. R. TenHuisen, Preston Zhou, Sunwook Park, Hoon Kim, Jin-Kwang Kim, Hyeong-Do Kim, Minseok Kim, Sang‐Youn Park, Peter Abbamonte, Genda Gu, Yao Wang, Matteo Mitrano

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePhysical Review X · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPhysics of Superconductivity and Magnetism
Canadian institutionsUniversity of British Columbia
FundersBasic Energy SciencesMinistry of Science and ICT, South KoreaSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungCanada First Research Excellence FundOffice of ScienceUniversity of TokyoNational Research FoundationInstitute for Basic ScienceNational Energy Research Scientific Computing CenterNational Research Foundation of KoreaGordon and Betty Moore FoundationBrookhaven National LaboratoryU.S. Department of EnergyHarvard UniversityNational Science Foundation
KeywordsCuprateSuperconductivityRenormalizationCoulombPhysicsUltrashort pulseCondensed matter physicsQuantum mechanicsElectron

Abstract

fetched live from OpenAlex

Ultrafast lasers are an increasingly important tool to control and stabilize emergent phases in quantum materials. Among a variety of possible excitation protocols, a particularly intriguing route is the direct light engineering of microscopic electronic parameters, such as the electron hopping and the local Coulomb repulsion (Hubbard U). In this work, we use time-resolved x-ray absorption spectroscopy to demonstrate the light-induced renormalization of the Hubbard U in a cuprate superconductor, La 1.905 Ba 0.095 CuO 4 . We show that intense femtosecond laser pulses induce a substantial redshift of the upper Hubbard band while leaving the Zhang-Rice singlet energy unaffected. By comparing the experimental data to time-dependent spectra of single-and three-band Hubbard models, we assign this effect to an approximately 140-meV reduction of the on-site Coulomb repulsion on the copper sites. Our demonstration of a dynamical Hubbard U renormalization in a copper oxide paves the way to a novel strategy for the manipulation of superconductivity and magnetism as well as to the realization of other long-range-ordered phases in light-driven quantum materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: Theoretical or conceptual
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.213
Threshold uncertainty score0.595

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.269
Teacher spread0.257 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it