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Record W4226025792 · doi:10.1155/2022/1924117

Adsorption of Phenol onto Aluminum Oxide Nanoparticles: Performance Evaluation, Mechanism Exploration, and Principal Component Analysis (PCA) of Thermodynamics

2022· article· en· W4226025792 on OpenAlexaff
Safwat M. Safwat, Nouran Y. Mohamed, Mohamed N.A. Meshref, Abdelsalam Elawwad

Bibliographic record

VenueAdsorption Science & Technology · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsAdsorptionChemistryAqueous solutionEndothermic processPhenolNanoparticleExothermic reactionLangmuir adsorption modelDiffusionOxideChemical engineeringLangmuirInorganic chemistryThermodynamicsOrganic chemistry

Abstract

fetched live from OpenAlex

The removal of phenolic compounds from aqueous solutions using novel adsorption techniques becomes a key research item. Of those, nanoparticles in particular, the low-cost and the high-strength aluminum oxide nanoparticles showed promising results in pollutant uptake and increase in the adsorption efficiency. This study examined various physicochemical process parameters such as temperature, pH, initial phenol concentration, and adsorbent doses, in addition to the impact of those parameters on the adsorption removal mechanism of phenol. The results highlighted that aluminum oxide nanoparticles successfully exhibited superior phenol removal from an aqueous solution in addition to a high potential regeneration of the consumed nanoparticles by HCl. For the adsorbent mass of 0.5 g, phenol adsorption uptake reached 92%. Kinetic studies performed using several models demonstrated the data best fitting with a pseudo-second-order kinetic model. Examining equilibrium studies of various isotherms, the adsorption data of phenol into aluminum oxide nanoparticles was confirmed to be controlled by film diffusion and best represented by the Langmuir isotherm. The maximum capacity of adsorption was 16.97 mg/g. For thermodynamics studies, the results indicated that the adsorption process can vary between endothermic and exothermic reactions. Such relative differences in heat generation and spontaneity in adsorption processes were demonstrated and confirmed by principal component analysis (PCA). This evidence is key for future investigations for the efficiency of adsorption conditions concerning the contaminant type and adsorbate compounds.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.251
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2022
Admission routes1
Has abstractyes

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Same venueAdsorption Science & TechnologySame topicAdsorption and biosorption for pollutant removalFrench-language works237,207