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Record W4229372131 · doi:10.26434/chemrxiv-2022-b3f72

Comparing corrosion control treatments using a robust Bayesian generalized additive model

2022· preprint· en· W4229372131 on OpenAlexafffund
Benjamin F. Trueman, Wendell James, Trevor Shu, Evelyne Doré, Graham A. Gagnon

Bibliographic record

VenueChemRxiv · 2022
Typepreprint
Languageen
FieldEnvironmental Science
TopicWater Quality Monitoring and Analysis
Canadian institutionsDalhousie University
FundersNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsOverfittingBayesian probabilityOutlierAutocorrelationNonlinear autoregressive exogenous modelStatistical hypothesis testingBayesian inferenceAutoregressive modelRank (graph theory)Computer scienceStatisticsData miningMathematicsArtificial intelligenceArtificial neural network

Abstract

fetched live from OpenAlex

Pipe loop studies are used routinely to evaluate corrosion control treatment, and updated regulatory guidance will ensure that they remain an important tool for water quality management. But they are inherently complex and the data they generate are difficult to analyze: non-linear time-trends, non-detects, extreme values, and autocorrelation are common features, the latter due to repeatedly measuring the effluent from test pipes. Popular statistical tests, such as the Student t or rank-sum tests, are often inadequate descriptions of the data. Here, we propose an approach to statistical analysis of pipe loop data that accommodates many of these difficult-to-model characteristics: a robust Bayesian generalized additive model with continuous-time autoregressive errors. Our model facilitates corrosion control treatment comparisons without the need for imputing non-detects or special handling of outliers. It is well-suited to describing nonlinear trends without overfitting, and it accounts for reduced information content due to autocorrelation. We demonstrate the model using an example pipe loop study comprising four years of data, multiple pipe configurations, and multiple orthophosphate dosing protocols. We compare the experimental treatments, finding that an initially high dose of orthophosphate (2 mg P L-1) that is subsequently lowered (0.75 mg P L-1) can yield lower lead release than an intermediate dose (1 mg P L-1) in the long term. We also find that—consistent with previous work—galvanic corrosion yields relatively high particulate lead release, especially at higher orthophosphate doses. An advantage of the Bayesian approach we adopt here is that it yields the full posterior distribution of all parameters and all quantities derived from those parameters, including the model predictions. This means that analysts can construct any comparison that is relevant to the study goals, without the need to rely on a particular statistical test.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.033
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.074
GPT teacher head0.283
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2022
Admission routes2
Has abstractyes

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