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Record W4230508477 · doi:10.32920/ryerson.14647803

Novel modified QAC antimicrobial coatings: application, evaluation and functional determination

2021· preprint· en· W4230508477 on OpenAlexaff
Alexander Gabriel Caschera

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldChemistry
TopicAntimicrobial agents and applications
Canadian institutionsToronto Metropolitan University
Fundersnot available
KeywordsAlkylAntimicrobialAmmoniumAnchoringArylChemistrySulfonamideBenzophenoneHomologous seriesBacteriaStereochemistryCombinatorial chemistryPolymer chemistryMaterials scienceOrganic chemistryBiology

Abstract

fetched live from OpenAlex

A series of novel quaternary ammonium compounds (QACs) previously synthesized by the Foucher Research Group containing the core motif R1-(CH2)3-N+ (CH3)2-(CH2)3-R2, where R1 represents functional groups responsible for anchoring the compound to various substrates and R2 represents moieties responsible for altering the activity and surface properties of coated materials are described. R1 groups include benzophenone (-O-C6H4-C(O)-C6H5) 1a-11a for anchoring to polymer surfaces, and organosilane (-Si(OCH3) 3b-10b for anchoring to textiles and fabrics, while R2 groups include linear alkyl chains (-(CH2)n-CH3; n = 11, 17) 1-2 and aryl or alkyl sulfonamide containing moieties (-NH-SO2-CXHY, x = 2-10; y = 5-11) 3-11. These compounds were tested for antimicrobial activity at solid/air interfaces (LDI) and were found highly effective against representative Gram-positive and Gram-negative bacteria (except 7a-8a, 11a). Selective solid/liquid antimicrobial testing (LRI) was performed on 1a, 5a and only 5a was found to be highly effective against Gram-positive bacteria.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.559
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.037
GPT teacher head0.283
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2021
Admission routes1
Has abstractyes

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