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Record W4233157928 · doi:10.1002/ange.200800721

Sulfated Mesoporous Tantalum Oxides in the Shape Selective Synthesis of Linear Alkyl Benzene

2008· article· en· W4233157928 on OpenAlexaff
Junjie Kang, Yuxiang Rao, Michel L. Trudeau, David M. Antonelli

Bibliographic record

VenueAngewandte Chemie · 2008
Typearticle
Languageen
FieldChemistry
TopicZeolite Catalysis and Synthesis
Canadian institutionsHydro-QuébecUniversity of Windsor
Fundersnot available
KeywordsChemistryBenzeneAlkylMesoporous materialMedicinal chemistryStereochemistryCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Gut gerüstet: Mesoporöse Tantaloxide wurden mit 1.0 M Schwefelsäure behandelt und auf ihre katalytische Aktivität und Selektivität in der Synthese von 2-Phenylisomeren durch Alkylierung von Benzol mit sperrigen Olefinen getestet (siehe Schema). Das sulfatierte mesoporöse Tantaloxid zeigte ähnliche Aktivitäten wie Zeolith HY, bei jedoch sehr viel höherer Selektivität für 2-Phenyldodecan unter milden Bedingungen. Die hohe Aktivität und Selektivität wird durch die erleichterte Diffusion von sperrigen Reaktanten in den mesoporösen Gerüsten erklärt. Supporting information for this article is available on the WWW under http://www.wiley-vch.de/contents/jc_2001/2008/z800721_s.pdf or from the author. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.029
Threshold uncertainty score0.820

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.234
Teacher spread0.212 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2008
Admission routes1
Has abstractyes

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