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Record W4233887831 · doi:10.22215/etd/2017-12065

Synthesis and Luminescent Properties of Graphene Quantum Dots (GQDs) for Fluorescence Quenching by Titanium Dioxide Nanoparticles in Water Analysis

2017· dissertation· en· W4233887831 on OpenAlexaff
Kaiyu Wang

Bibliographic record

Venuenot available
Typedissertation
Languageen
FieldMaterials Science
TopicCarbon and Quantum Dots Applications
Canadian institutionsCarleton University
Fundersnot available
KeywordsGrapheneTitanium dioxideQuenching (fluorescence)NanoparticleMaterials scienceQuantum dotFluorescenceLuminescenceOxideNanotechnologyChemical engineeringOptoelectronicsComposite material

Abstract

fetched live from OpenAlex

Graphene quantum dots (GQDs) have many excellent properties such as strong fluorescence, chemical stability and facile synthesis. In this work, GQDs were prepared by pyrolysis of citric acid. And optimization of the pyrolysis temperature, pyrolysis time, and dispersion pH attained 1.04 times stronger fluorescence intensity.The appearance of metal oxide nanoparticles in potable water has attracted much public attention. A simple method for quantitative analysis of titanium dioxide (TiO2) nanoparticles was developed by fluorescence quenching of GQDs in this research. Dopamine (DA) was first added to coat TiO2 nanoparticles with polydopamine (PDA) under ultrasonication. GQDs were next added as a fluorescent sensor probe to measure the quenching of its emission intensity by the PDA-coated nanoparticles. Data analysis by the Stern-Volmer equation followed a third-order polynomial fit that indicated static, dynamic and absorptive contributions to the total quenching. Detection of TiO2 nanoparticles down to 0.02 mg/mL was validated.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.642

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.257
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2017
Admission routes1
Has abstractyes

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