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Record W4237660588 · doi:10.1021/bk-2000-0752.ch026

A Novel Composite Membrane for Temperature-and pH-Responsive Permeation

2000· book-chapter· en· W4237660588 on OpenAlexafffund
F. Yam, Xiao Yu Wu, Qiuping Zhang

Bibliographic record

VenueACS symposium series · 2000
Typebook-chapter
Languageen
FieldEngineering
TopicElectrochemical sensors and biosensors
Canadian institutionsUniversity of Toronto
FundersMedical Research CouncilNatural Sciences and Engineering Research Council of Canada
KeywordsPermeationMembraneChemical engineeringNanoparticlePermeability (electromagnetism)Methacrylic acidPolymerChemistryChromatographyMaterials scienceOrganic chemistryMonomer

Abstract

fetched live from OpenAlex

A stimuli-sensitive composite membrane was prepared from nanoparticles of poly(N-isopropylacrylamide-co-methacrylic acid) and a hydrophobic polymer. The effects of temperature, solute size, and pH on the solute permeation through the membrane were studied. The permeation rate increased with increasing temperature or decreasing pH. A greater increase was found for larger molecules like vitamin B12 than smaller ones. Both membrane hydration and solute partition, decreasing with increasing temperature, could not explain the increased permeability. Thus a gel-pore mechanism of permeation was proposed that the solutes could diffuse through the membrane via two pathways, namely the gel phase of the nanoparticles and the water-filled pores, depending upon the molecular size. The nanoparticles acted as nanovalves controlling the pore size of the membrane by their volume change. The SEM photographs evidenced the porous structure of the membrane when the nanoparticles collapsed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.166
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.184
Teacher spread0.178 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2000
Admission routes2
Has abstractyes

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