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Record W4238968734 · doi:10.5194/acpd-14-29331-2014

The POLARCAT Model Intercomparison Project (POLMIP): overview and evaluation with observations

2014· preprint· en· W4238968734 on OpenAlexaboutno aff
L. K. Emmons, S. R. Arnold, S. A. Monks, Vincent Huijnen, Simone Tilmes, Kathy S. Law, Jennie L. Thomas, Jean‐Christophe Raut, Idir Bouarar, Solène Turquéty, Y. Long, B. N. Duncan, Stephen D. Steenrod, Sarah A. Strode, Johannes Flemming, Jingqiu Mao, Joakim Langner, Anne M. Thompson, D. W. Tarasick, Eric C. Apel, D. R. Blake, R. C. Cohen, Jack E. Dibb, Glenn S. Diskin, Alan Fried, Samuel R. Hall, L. G. Huey, A. J. Weinheimer, Armin Wisthaler, Tomáš Mikoviny, J. B. Nowak, Jeff Peischl, J. M. Roberts, Thomas B. Ryerson, C. Warneke, Detlev Helmig

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsnot available
Fundersnot available
KeywordsEnvironmental scienceAtmospheric sciencesChemical transport modelAcetaldehydeMeteorologyAtmospheric chemistryClimatologyEmission inventoryAerosolOzoneChemistryAir quality indexGeography

Abstract

fetched live from OpenAlex

Abstract. A model intercomparison activity was inspired by the large suite of atmospheric chemistry observations made during the International Polar Year (2008) in the Arctic. Nine global and two regional chemical transport models have performed simulations for 2008 using a common emissions inventory to quantify the differences in model chemistry and transport schemes. This paper summarizes the models and compares their simulations of ozone and its precursors, and presents an evaluation of the simulations using a variety of surface, balloon, aircraft and satellite observations. Despite using the same emissions, large differences are seen among the models. Differences in a number of model parameters are identified as contributing to differences in the modelled chemical species, including cloud fields and photolysis rates. The largest differences among models, and between models and observations, are in NOy partitioning (PAN vs. HNO3) and in oxygenated volatile organic compounds (VOCs) such as acetaldehyde and acetone. Comparisons to surface site measurements of ethane and propane indicate that the emissions of these species are significantly underestimated. While limited in spatial and temporal coverage, the aircraft measurements provide a simultaneous evaluation of many species. Satellite observations of NO2 from OMI have been used to evaluate the models over source regions, indicating anthropogenic emissions are underestimated in East Asia, but fire emissions are generally overestimated. The emission factors for wildfires in Canada are evaluated using the correlations of VOCs to CO in the model output in comparison to enhancement factors derived from aircraft observations, showing reasonable agreement for methanol and acetaldehyde, but underestimate of ethanol, propane and acetone, while overestimating ethane emission factors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.009
metaresearch head score (Gemma)0.006
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.038
Threshold uncertainty score0.075

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0090.006
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.002
Science and technology studies0.0010.000
Scholarly communication0.0020.002
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.113
GPT teacher head0.302
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2014
Admission routes1
Has abstractyes

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