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Record W4245503810 · doi:10.31224/osf.io/q7v9r

Functionalization of metal Nanoparticles for SERS-based Detections of illicit drugs in biological samples

2020· preprint· en· W4245503810 on OpenAlexaff
Shamim Azimi

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldMaterials Science
TopicGold and Silver Nanoparticles Synthesis and Applications
Canadian institutionsQueen's University
Fundersnot available
KeywordsSurface modificationNanotechnologyRaman scatteringAnalyteNanoparticleMaterials sciencePlasmonSubstrate (aquarium)Computer scienceRaman spectroscopyChemistryChromatographyOptoelectronicsOptics

Abstract

fetched live from OpenAlex

Surface-enhanced Raman scattering (SERS) has been widely used for the detection of illicit drugs due to its excellent chemical fingerprint information, high sensitivity by plasmon-enhanced excitation and scattering, and independence of aqueous solution impact. Even though it has been more than one decade since the first SERS was synthesized, extensive effort has recently been undertaken to improve hand-held Raman analyzer and make SERS a practical point-of-care (POC) device for the detection of illicit drugs in real samples. Lately, there has been a fast growth in improving methods for precise control over metal nanoparticle size and modification of their detection performance with functionalizing agents, which will dramatically enhance their application in various biomedical applications.In this study, a general view on the background of the SERS and several basic concepts and focuses are discussed. Then we put forward a summary of the progress in trace determination of illicit drugs using various functionalization methods for enhancing characteristics of the substrate toward a more selective detection of the analytes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.080
GPT teacher head0.283
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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